Samset Bjørn H, Stjern Camilla W, Andrews Elisabeth, Kahn Ralph A, Myhre Gunnar, Schulz Michael, Schuster Gregory L
CICERO Center for International Climate Research, Oslo, Norway.
2CIRES, University of Colorado, Boulder, CO USA.
Curr Clim Change Rep. 2018;4(2):65-83. doi: 10.1007/s40641-018-0091-4. Epub 2018 Apr 3.
Some aerosols absorb solar radiation, altering cloud properties, atmospheric stability and circulation dynamics, and the water cycle. Here we review recent progress towards global and regional constraints on aerosol absorption from observations and modeling, considering physical properties and combined approaches crucial for understanding the total (natural and anthropogenic) influences of aerosols on the climate.
We emphasize developments in black carbon absorption alteration due to coating and ageing, brown carbon characterization, dust composition, absorbing aerosol above cloud, source modeling and size distributions, and validation of high-resolution modeling against a range of observations.
Both observations and modeling of total aerosol absorption, absorbing aerosol optical depths and single scattering albedo, as well as the vertical distribution of atmospheric absorption, still suffer from uncertainties and unknowns significant for climate applications. We offer a roadmap of developments needed to bring the field substantially forward.
一些气溶胶吸收太阳辐射,改变云的特性、大气稳定性和环流动力学以及水循环。在此,我们回顾了近期在通过观测和建模对气溶胶吸收进行全球和区域限制方面取得的进展,同时考虑了对于理解气溶胶对气候的总体(自然和人为)影响至关重要的物理特性和综合方法。
我们着重介绍了因包覆和老化导致的黑碳吸收变化、棕碳特征、沙尘成分、云上方吸收性气溶胶、源建模和粒径分布方面的进展,以及针对一系列观测对高分辨率建模的验证。
对于总气溶胶吸收、吸收性气溶胶光学厚度和单次散射反照率的观测和建模,以及大气吸收的垂直分布,在气候应用方面仍存在重大的不确定性和未知因素。我们提供了使该领域取得实质性进展所需的发展路线图。