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室内空气和不同沙特微观环境灰尘样本中的多环芳烃(PAHs);一般人群的健康和致癌风险评估。

Polycyclic aromatic hydrocarbons (PAHs) in indoor air and dust samples of different Saudi microenvironments; health and carcinogenic risk assessment for the general population.

机构信息

Center of Excellence in Environmental Studies, King Abdulaziz University, Saudi Arabia.

出版信息

Sci Total Environ. 2019 Dec 15;696:133995. doi: 10.1016/j.scitotenv.2019.133995. Epub 2019 Aug 20.

Abstract

In this study, the presence of polycyclic aromatic hydrocarbons (PAHs) was studied in indoor air (PM10) and settled dust collected from different indoor microenvironments of Saudi Arabia. Limited data is available on the indoor quality of Saudi Arabia and to the best of our knowledge, this is the first study reporting PAHs in indoor air from Saudi Arabia. The main objectives were to study the levels and profile of selected PAHs in indoor dust and PM10 samples from different microenvironments of Saudi Arabia and to estimate health risk assessment to the local population via inhalation, dust ingestion and dermal contact. To study PAHs, indoor dust and PM10 samples were collected from different households, offices and hotel roomsPM10.Pyrene, benz(a)anthracene, chrysene, and phenanthrene were the major PAHs in both settled dust and PM10 samples. Profile of PAHs in dust samples was dominated by 3 and 4 ring PAHs while in PM10 sample 5-6 aromatic ring PAHs also contributed significantly. PM10 collected from kitchens and AC filter dust samples were the most contaminated with PAHs. PM10Health risk assessment was made for adults and young based on benzo(a)pyrene equivalent carcinogenic power (BaPE) and incremental lifetime cancer risk (ILCR). BaPE revealed major toxicity threat associated with PAHs is all microenvironments samples (dust and PM10) is from 5 and 6 aromatic rings PAHs. ILRC calculated using ingestion, inhalation and dermal contact was within the limits set by USEPA and although using max concentration it was up to 8.0E-05, which can have significant impact long term if other exposure pathways such as food and outdoor exposure, etc. are considered.

摘要

在这项研究中,研究了室内空气(PM10)和从沙特阿拉伯不同室内微环境中收集的沉降灰尘中多环芳烃(PAHs)的存在。关于沙特阿拉伯室内空气质量的可用数据有限,据我们所知,这是首次报道沙特阿拉伯室内空气中多环芳烃的研究。主要目的是研究沙特阿拉伯不同微环境中室内灰尘和 PM10 样品中选定的多环芳烃的水平和特征,并通过吸入、灰尘摄入和皮肤接触来估计对当地居民的健康风险评估。为了研究多环芳烃,从不同家庭、办公室和酒店房间采集了室内灰尘和 PM10 样品。在沉降灰尘和 PM10 样品中,苊、苯并(a)蒽、屈和菲是主要的多环芳烃。灰尘样品中多环芳烃的特征是 3 环和 4 环多环芳烃,而 PM10 样品中 5-6 个芳香环多环芳烃也有显著贡献。从厨房和空调过滤器收集的 PM10 灰尘样品中含有最多的多环芳烃。根据苯并(a)芘等效致癌能力(BaPE)和增量终身癌症风险(ILCR),对成人和儿童进行了 PM10 健康风险评估。BaPE 显示,所有微环境样品(灰尘和 PM10)中与多环芳烃相关的主要毒性威胁来自 5 环和 6 环多环芳烃。通过摄入、吸入和皮肤接触计算的 ILRC 在 USEPA 设定的范围内,尽管使用最大浓度,其值高达 8.0E-05,如果考虑到其他暴露途径,如食物和室外暴露等,可能会对长期产生重大影响。

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