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受工业企业分布影响的土壤重金属的空间分布与来源分析:以江苏省为例。

Spatial distribution and source analysis of heavy metals in soils influenced by industrial enterprise distribution: Case study in Jiangsu Province.

机构信息

Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China; College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China; Key Laboratory of Watershed Geographic Sciences, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China.

Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China; Key Laboratory of Watershed Geographic Sciences, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China.

出版信息

Sci Total Environ. 2020 Mar 25;710:134953. doi: 10.1016/j.scitotenv.2019.134953. Epub 2019 Dec 3.

Abstract

Heavy metal pollution is frequent in China and has received increasing attention globally. This study investigated the influence of Chinese industrialization and urbanization on soil environmental quality. Soil samples from Jiangsu Province were collected, the Cd, Pb, Cr, Cu, Zn, Hg, and As contents were measured, and their spatial variability structure, spatial distribution pattern, and pollution degree were analyzed. The mean values of Hg, Cd, Pb, Cr, Cu, and As were all higher than the background values in Jiangsu Province. Cr and As levels represented moderate pollution, Cu, Zn, Cd, and Pb represented mild pollution, Cr and As represented slight pollution, and Hg was not a pollutant. Spatial distribution patterns were both zonal and concentrated in nature. High concentrations of heavy metals were distributed in developed cities and industrial parks along the Yangtze River. Soil heavy metal pollution showed a decreasing trend from south to north, consistent with the economic gradient. Industrialization had the greatest influence on the spatial heterogeneity of heavy metal pollution. Cr, Cu, Zn, and As were affected by both natural and anthropogenic sources, while Cd and Pb were mainly affected by the latter. Hg was mainly derived from industrial activities such as petrochemical production. There was spatial consistency between industrial enterprise distribution and soil heavy metal pollution with a tendency toward composite pollution accumulated by multiple elements in the soil surrounding industries.

摘要

重金属污染在中国很常见,已受到全球越来越多的关注。本研究探讨了中国工业化和城市化对土壤环境质量的影响。采集了江苏省的土壤样本,测量了 Cd、Pb、Cr、Cu、Zn、Hg 和 As 的含量,并分析了其空间变异性结构、空间分布模式和污染程度。Hg、Cd、Pb、Cr、Cu 和 As 的平均值均高于江苏省的背景值。Cr 和 As 水平代表中度污染,Cu、Zn、Cd 和 Pb 代表轻度污染,Cr 和 As 代表轻微污染,Hg 不是污染物。空间分布模式既有地带性又有集中性。重金属的高浓度分布在长江沿岸发达城市和工业园区。土壤重金属污染从南到北呈递减趋势,与经济梯度一致。工业化对重金属污染的空间异质性影响最大。Cr、Cu、Zn 和 As 既受自然源又受人源影响,而 Cd 和 Pb 主要受后者影响。Hg 主要来自石化生产等工业活动。工业企业分布与土壤重金属污染之间存在空间一致性,工业周边土壤中多种元素复合污染有累积的趋势。

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