Cai Shuang, Deng Yingnan, Fu Shengnan, Li Junjie, Yu Changyuan, Su Xin
College of Life Science and Technology , Beijing University of Chemical Technology , Beijing 100029 , China . Email:
Chem Sci. 2019 Oct 7;10(43):9922-9927. doi: 10.1039/c9sc03389k. eCollection 2019 Nov 21.
DNA molecular switches have emerged as a versatile and highly programmable toolbox and are extensively used in sensing, diagnosis, and therapeutics. Toehold mediated strand displacement serves as the core reaction for signal transduction and amplification. However, the severe leakage of this reaction limits the development of scalable and robust circuits. We engineered single-molecule dynamic DNA junctions for developing 'zero-leakage' molecular switches which are responsive to various inputs. Input binding enhances dynamic junctions' stability allowing for the transient binding of fluorescent probes as the output signal. Unlike the conventional intensity-based output, this molecular switch provides remarkably distinguishable kinetics-based outputs permitting ruling out leakage signals at the single-molecule level. The inputs are detected with significant sensitivity without using any amplification step. It is also revealed that the output signal is sensitive to the binding affinity of inputs and their recognition elements making the molecular switch a potential affinity meter. Considering these features, we anticipate that it would find broad applications in large-scale DNA circuits, responsive materials, and biomolecule interaction study.
DNA分子开关已成为一种多功能且高度可编程的工具箱,并广泛应用于传感、诊断和治疗领域。托住介导的链置换作为信号转导和放大的核心反应。然而,该反应的严重泄漏限制了可扩展且稳健的电路的发展。我们设计了单分子动态DNA连接体,以开发对各种输入有响应的“零泄漏”分子开关。输入结合增强了动态连接体的稳定性,使得荧光探针能够作为输出信号进行瞬时结合。与传统的基于强度的输出不同,这种分子开关提供了基于动力学的显著可区分输出,从而能够在单分子水平上排除泄漏信号。在不使用任何放大步骤的情况下,能够以显著的灵敏度检测输入。研究还表明,输出信号对输入及其识别元件的结合亲和力敏感,这使得分子开关成为一种潜在的亲和力测量仪。考虑到这些特性,我们预计它将在大规模DNA电路、响应材料和生物分子相互作用研究中得到广泛应用。