Hassanpouryouzband Aliakbar, Joonaki Edris, Edlmann Katriona, Heinemann Niklas, Yang Jinhai
School of Geosciences, University of Edinburgh, Grant Institute, West Main Road, Edinburgh, EH9 3JW, UK.
TÜV SÜD National Engineering Laboratory, Scottish Enterprise Technology Park, East Kilbride, South Lanarkshire, G75 0QF, United Kingdom.
Sci Data. 2020 Jul 9;7(1):222. doi: 10.1038/s41597-020-0568-6.
The use of hydrogen (H) as a substitute for fossil fuel, which accounts for the majority of the world's energy, is environmentally the most benign option for the reduction of CO emissions. This will require gigawatt-scale storage systems and as such, H storage in porous rocks in the subsurface will be required. Accurate estimation of the thermodynamic and transport properties of H mixed with other gases found within the storage system is therefore essential for the efficient design for the processes involved in this system chain. In this study, we used the established and regarded GERG-2008 Equation of State (EoS) and SuperTRAPP model to predict the thermo-physical properties of H mixed with CH, N, CO, and a typical natural gas from the North-Sea. The data covers a wide range of mole fraction of H (10-90 Mole%), pressures (0.01-100 MPa), and temperatures (200-500 K) with high accuracy and precision. Moreover, to increase ease of access to the data, a user-friendly software (H2Themobank) is developed and made publicly available.
使用氢气(H)替代占全球能源大部分的化石燃料,在减少二氧化碳排放方面是对环境最为有利的选择。这将需要千兆瓦规模的存储系统,因此需要将氢气存储在地下多孔岩石中。准确估算存储系统中氢气与其他气体混合时的热力学和传输特性,对于该系统链所涉及过程的高效设计至关重要。在本研究中,我们使用已确立且受认可的GERG - 2008状态方程(EoS)和SuperTRAPP模型,来预测氢气与甲烷、氮气、一氧化碳以及一种来自北海的典型天然气混合时的热物理性质。数据涵盖了氢气的广泛摩尔分数范围(10% - 90%摩尔分数)、压力范围(0.01 - 100兆帕)以及温度范围(200 - 500开尔文),具有高精度和高精确度。此外,为了更方便地获取这些数据,还开发了一个用户友好型软件(H2Themobank)并公开发布。