Laatiaoui Mustapha, Buchachenko Alexei A, Viehland Larry A
Department Chemie, Johannes Gutenberg-Universität, Fritz-Strassmann Weg 2, 55128 Mainz, Germany.
Helmholtz-Institut Mainz, Staudingerweg 18, 55128 Mainz, Germany.
Phys Rev Lett. 2020 Jul 10;125(2):023002. doi: 10.1103/PhysRevLett.125.023002.
Optical spectroscopy constitutes the historical path to accumulate basic knowledge on the atom and its structure. Former work based on fluorescence and resonance ionization spectroscopy enabled identifying optical spectral lines up to element 102, nobelium. The new challenges faced in this research field are the refractory nature of the heavier elements and the decreasing production yields. A new concept of ion-mobility-assisted laser spectroscopy is proposed to overcome the sensitivity limits of atomic structure investigations persisting in the region of the superheavy elements. The concept offers capabilities of both broadband-level searches and high-resolution hyperfine spectroscopy of synthetic elements beyond nobelium.
光谱学是积累关于原子及其结构的基础知识的历史途径。以前基于荧光和共振电离光谱的工作能够识别出直至102号元素锘的光谱线。该研究领域面临的新挑战是超重元素的难熔性质以及产量的下降。提出了一种离子迁移辅助激光光谱的新概念,以克服在超重元素区域持续存在的原子结构研究的灵敏度限制。该概念提供了对锘以后的合成元素进行宽带水平搜索和高分辨率超精细光谱分析的能力。