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金属性受挫磁体候选材料KVSb中的巨大非常规反常霍尔效应

Giant, unconventional anomalous Hall effect in the metallic frustrated magnet candidate, KVSb.

作者信息

Yang Shuo-Ying, Wang Yaojia, Ortiz Brenden R, Liu Defa, Gayles Jacob, Derunova Elena, Gonzalez-Hernandez Rafael, Šmejkal Libor, Chen Yulin, Parkin Stuart S P, Wilson Stephen D, Toberer Eric S, McQueen Tyrel, Ali Mazhar N

机构信息

Max Planck Institute of Microstructure Physics, Halle, Germany.

University of California at Santa Barbara, Santa Barbara, California 93106, USA.

出版信息

Sci Adv. 2020 Jul 31;6(31):eabb6003. doi: 10.1126/sciadv.abb6003. eCollection 2020 Jul.

Abstract

The anomalous Hall effect (AHE) is one of the most fundamental phenomena in physics. In the highly conductive regime, ferromagnetic metals have been the focus of past research. Here, we report a giant extrinsic AHE in KVSb, an exfoliable, highly conductive semimetal with Dirac quasiparticles and a vanadium Kagome net. Even without report of long range magnetic order, the anomalous Hall conductivity reaches 15,507 Ω cm with an anomalous Hall ratio of ≈ 1.8%; an order of magnitude larger than Fe. Defying theoretical expectations, KVSb shows enhanced skew scattering that scales quadratically, not linearly, with the longitudinal conductivity, possibly arising from the combination of highly conductive Dirac quasiparticles with a frustrated magnetic sublattice. This allows the possibility of reaching an anomalous Hall angle of 90° in metals. This observation raises fundamental questions about AHEs and opens new frontiers for AHE and spin Hall effect exploration, particularly in metallic frustrated magnets.

摘要

反常霍尔效应(AHE)是物理学中最基本的现象之一。在高导电状态下,铁磁金属一直是过去研究的重点。在此,我们报道了在KVSb中发现的巨大的外在反常霍尔效应,KVSb是一种可剥离的、具有狄拉克准粒子和钒 Kagome 网的高导电半金属。即使没有长程磁有序的报道,反常霍尔电导率仍达到15507Ω·cm,反常霍尔比约为1.8%;比铁大一个数量级。与理论预期相反,KVSb显示出增强的斜散射,其与纵向电导率呈二次方而非线性关系,这可能源于高导电狄拉克准粒子与受挫磁亚晶格的结合。这使得在金属中达到90°的反常霍尔角成为可能。这一观察结果引发了关于反常霍尔效应的基本问题,并为反常霍尔效应和自旋霍尔效应的探索开辟了新的前沿领域,特别是在金属受挫磁体中。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b868/7399694/a0f410275785/abb6003-F1.jpg

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