Weber James, Shin Youngsub M, Staunton Sykes John, Archer-Nicholls Scott, Abraham N Luke, Archibald Alex T
Centre for Atmospheric Science, Department of Chemistry University of Cambridge Cambridge UK.
National Centre for Atmospheric Science, Department of Chemistry University of Cambridge Cambridge UK.
Geophys Res Lett. 2020 Oct 28;47(20):e2020GL090326. doi: 10.1029/2020GL090326. Epub 2020 Oct 22.
We present an assessment of the impacts on atmospheric composition and radiative forcing of short-lived pollutants following a worldwide decrease in anthropogenic activity and emissions comparable to what has occurred in response to the COVID-19 pandemic, using the global composition-climate model United Kingdom Chemistry and Aerosols Model (UKCA). Emission changes reduce tropospheric hydroxyl radical and ozone burdens, increasing methane lifetime. Reduced SO emissions and oxidizing capacity lead to a decrease in sulfate aerosol and increase in aerosol size, with accompanying reductions to cloud droplet concentration. However, large reductions in black carbon emissions increase aerosol albedo. Overall, the changes in ozone and aerosol direct effects (neglecting aerosol-cloud interactions which were statistically insignificant but whose response warrants future investigation) yield a radiative forcing of -33 to -78 mWm. Upon cessation of emission reductions, the short-lived climate forcers rapidly return to pre-COVID levels; meaning, these changes are unlikely to have lasting impacts on climate assuming emissions return to pre-intervention levels.
我们使用全球成分-气候模型英国化学和气溶胶模型(UKCA),评估了在全球范围内人为活动和排放减少程度与应对新冠疫情时相当的情况下,短寿命污染物对大气成分和辐射强迫的影响。排放变化减少了对流层羟基自由基和臭氧负担,增加了甲烷寿命。二氧化硫排放和氧化能力的降低导致硫酸盐气溶胶减少和气溶胶粒径增大,同时云滴浓度降低。然而,黑碳排放的大幅减少增加了气溶胶反照率。总体而言,臭氧和气溶胶直接效应的变化(忽略气溶胶-云相互作用,其在统计上不显著,但其响应值得未来研究)产生的辐射强迫为-33至-78毫瓦/平方米。在减排停止后,短寿命气候强迫因子迅速恢复到新冠疫情前的水平;这意味着,假设排放恢复到干预前水平,这些变化不太可能对气候产生持久影响。