Institute of Reproductive and Child Health / Ministry of Health Key Laboratory of Reproductive Health and Department of Epidemiology and Biostatistics, School of Public Health, Peking University, Beijing 100191, China.
Ministry of Education Key Laboratory for Earth System Modeling, Department of Earth System Science, Tsinghua University, Beijing 100084, China.
Environ Sci Technol. 2020 Dec 1;54(23):14877-14888. doi: 10.1021/acs.est.0c03098. Epub 2020 Nov 11.
Since 2013, clean-air actions in China have reduced ambient concentrations of PM. However, recent studies suggest that ground surface O concentrations increased over the same period. To understand the shift in air pollutants and to comprehensively evaluate their impacts on health, a spatiotemporal model for O is required for exposure assessment. This study presents a data-fusion algorithm for O estimation that combines observations, satellite remote sensing measurements, and model results from the community multiscale air quality model. Performance of the algorithm for O estimation was evaluated by five-fold cross-validation. The estimates are highly correlated with the observations of the maximum daily 8 h averaged O ( = 0.70). The mean modeling error (measured using the root-mean-squared error) is 26 μg/m, which accounts for 29% of the mean level. We also found that satellite O played a key role to improve model performance, particularly during warm months. The estimates were further used to illustrate spatiotemporal variation in O during 2013-2017 for the whole country. In contrast to the reduced trend of PM, we found that the population-weighted O mean increased from 86 μg/m in 2013 to 95 μg/m in 2017, with a rate of 2.07 (95% CI: 1.65, 2.48) μg/m per year at the national level. This increased trend in O suggests that it is becoming an important contributor to the burden of diseases attributable to air pollutants in China. The developed method and the results generated from this study can be used to support future health-related studies in China.
自 2013 年以来,中国的清洁空气行动已经降低了环境中 PM 的浓度。然而,最近的研究表明,同期地面 O 的浓度有所上升。为了了解空气污染物的变化,并全面评估其对健康的影响,需要有一种用于暴露评估的 O 时空模型。本研究提出了一种用于 O 估算的数据融合算法,该算法结合了观测、卫星遥感测量和社区多尺度空气质量模型的模型结果。通过五重交叉验证评估了算法对 O 估算的性能。该估算值与每日 8 小时最大平均值 O 的观测值高度相关(=0.70)。平均建模误差(使用均方根误差测量)为 26μg/m,占平均值的 29%。我们还发现,卫星 O 在提高模型性能方面发挥了关键作用,尤其是在温暖的月份。这些估算值还被进一步用于说明 2013-2017 年期间全国范围内 O 的时空变化。与 PM 减少的趋势相反,我们发现,人口加权 O 的平均值从 2013 年的 86μg/m 增加到 2017 年的 95μg/m,全国水平每年增加 2.07(95%CI:1.65,2.48)μg/m。O 增加的趋势表明,它在中国空气污染物相关疾病负担中变得越来越重要。所开发的方法和本研究产生的结果可用于支持中国未来与健康相关的研究。