School of Physical Science and Technology, ShanghaiTech University, Shanghai, 201210, China.
University of Chinese Academy of Science, Beijing, 100049, China.
Angew Chem Int Ed Engl. 2021 Mar 1;60(10):5370-5376. doi: 10.1002/anie.202012720. Epub 2021 Jan 15.
We describe a cerium-catalyzed aerobic oxidative ring expansion for the expedient construction of synthetically challenging macrolactones under visible-light conditions. Cyanoanthracene has been employed as co-catalyst to accelerate the turnover of the cerium cycle leading to a fast conversion within 20 min of irradiation. Taking advantage of the high efficiency and operationally simple conditions, a collection of over 100 macrolactones equipped with ring systems ranging from 9- to 19-membered macrocycles have been prepared from simple building blocks. Moreover, the enabling potential of this strategy to simplify the generation of molecular complexity has been demonstrated through the concise synthesis of sonnerlactone.
我们描述了一种铈催化的有氧氧化环扩张反应,在可见光条件下,可快速构建具有挑战性的大环内酯。氰基蒽醌被用作共催化剂,以加速铈循环的周转,从而在辐照 20 分钟内实现快速转化。利用这种方法的高效率和操作简单的条件,我们从简单的起始原料出发,制备了超过 100 个大环内酯,其环系统的大小从 9 元到 19 元不等。此外,该策略在简化分子复杂性生成方面的应用潜力,通过简洁的索内内酯合成得到了证明。