Mohammadi Ershad, Tittl Andreas, Tsakmakidis Kosmas L, Raziman T V, Curto Alberto G
Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, 5600 MB Eindhoven, The Netherlands.
Chair in Hybrid Nanosystems, Nanoinstitute Munich, Faculty of Physics, Ludwig-Maximilians-Universität München, 80539 Munich, Germany.
ACS Photonics. 2021 Jun 16;8(6):1754-1762. doi: 10.1021/acsphotonics.1c00311. Epub 2021 May 28.
The discrimination of enantiomers is crucial in biochemistry. However, chiral sensing faces significant limitations due to inherently weak chiroptical signals. Nanophotonics is a promising solution to enhance sensitivity thanks to increased optical chirality maximized by strong electric and magnetic fields. Metallic and dielectric nanoparticles can separately provide electric and magnetic resonances. Here we propose their synergistic combination in hybrid metal-dielectric nanostructures to exploit their dual character for superchiral fields beyond the limits of single particles. For optimal optical chirality, in addition to maximization of the resonance strength, the resonances must spectrally coincide. Simultaneously, their electric and magnetic fields must be parallel and π/2 out of phase and spatially overlap. We demonstrate that the interplay between the strength of the resonances and these optimal conditions constrains the attainable optical chirality in resonant systems. Starting from a simple symmetric nanodimer, we derive closed-form expressions elucidating its fundamental limits of optical chirality. Building on the trade-offs of different classes of dimers, we then suggest an asymmetric dual dimer based on realistic materials. These dual nanoresonators provide strong and decoupled electric and magnetic resonances together with optimal conditions for chiral fields. Finally, we introduce more complex dual building blocks for a metasurface with a record 300-fold enhancement of local optical chirality in nanoscale gaps, enabling circular dichroism enhancement by a factor of 20. By combining analytical insight and practical designs, our results put forward hybrid resonators to increase chiral sensitivity, particularly for small molecular quantities.
对映体的鉴别在生物化学中至关重要。然而,由于固有手性光学信号较弱,手性传感面临重大限制。纳米光子学是一种很有前景的解决方案,可通过强电场和磁场使光学手性增加从而提高灵敏度。金属和介电纳米粒子可分别提供电共振和磁共振。在此,我们提出将它们协同组合在混合金属 - 介电纳米结构中,以利用其双重特性产生超越单个粒子极限的超手性场。为实现最佳光学手性,除了使共振强度最大化外,共振还必须在光谱上重合。同时,它们的电场和磁场必须平行且相位相差π/2 并在空间上重叠。我们证明共振强度与这些最佳条件之间的相互作用限制了共振系统中可实现的光学手性。从一个简单的对称纳米二聚体出发,我们推导出封闭形式的表达式,阐明其光学手性的基本极限。基于不同类型二聚体的权衡,我们随后提出一种基于实际材料的不对称双二聚体。这些双纳米谐振器提供强且解耦的电共振和磁共振以及手性场的最佳条件。最后,我们为超表面引入更复杂的双构建块,在纳米级间隙中实现局部光学手性创纪录的 300 倍增强,使圆二色性增强 20 倍。通过结合分析见解和实际设计,我们的结果提出了混合谐振器以提高手性灵敏度,特别是对于少量分子。