Wuhan National Laboratory for Optoelectronics and School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan, China.
Department of Electrical and Computer Engineering, National University of Singapore, Singapore, Singapore.
Nature. 2021 Aug;596(7872):362-366. doi: 10.1038/s41586-021-03755-1. Epub 2021 Aug 18.
Polaritons in anisotropic materials result in exotic optical features, which can provide opportunities to control light at the nanoscale. So far these polaritons have been limited to two classes: bulk polaritons, which propagate inside a material, and surface polaritons, which decay exponentially away from an interface. Here we report a near-field observation of ghost phonon polaritons, which propagate with in-plane hyperbolic dispersion on the surface of a polar uniaxial crystal and, at the same time, exhibit oblique wavefronts in the bulk. Ghost polaritons are an atypical non-uniform surface wave solution of Maxwell's equations, arising at the surface of uniaxial materials in which the optic axis is slanted with respect to the interface. They exhibit an unusual bi-state nature, being both propagating (phase-progressing) and evanescent (decaying) within the crystal bulk, in contrast to conventional surface waves that are purely evanescent away from the interface. Our real-space near-field imaging experiments reveal long-distance (over 20 micrometres), ray-like propagation of deeply subwavelength ghost polaritons across the surface, verifying long-range, directional and diffraction-less polariton propagation. At the same time, we show that control of the out-of-plane angle of the optic axis enables hyperbolic-to-elliptic topological transitions at fixed frequency, providing a route to tailor the band diagram topology of surface polariton waves. Our results demonstrate a polaritonic wave phenomenon with unique opportunities to tailor nanoscale light in natural anisotropic crystals.
各向异性材料中的极化激元会产生奇特的光学特性,这为在纳米尺度上控制光提供了机会。到目前为止,这些极化激元仅限于两类:在材料内部传播的体极化激元和从界面指数衰减的表面极化激元。在这里,我们报告了一种幽灵声子极化激元的近场观察结果,它在各向异性单轴晶体的表面上具有面内双曲色散传播,同时在体相表现出倾斜波前。幽灵极化激元是麦克斯韦方程组的一种非典型非均匀表面波解,出现在光轴相对于界面倾斜的单轴材料表面。它们表现出一种不寻常的双态性质,在晶体体相内部既是传播的(相位进展)又是渐逝的(衰减的),与传统的表面波不同,传统的表面波在离开界面时完全是渐逝的。我们的实空间近场成像实验揭示了深亚波长幽灵极化激元在表面上的远距离(超过 20 微米)、类似光线的传播,验证了长程、定向和无衍射的极化激元传播。同时,我们表明控制光轴的出射角能够在固定频率下实现双曲到椭圆的拓扑转变,为定制表面极化激波的能带图拓扑提供了一种途径。我们的结果展示了一种具有独特的纳米尺度光调控机会的极化激元波现象,在天然各向异性晶体中。