Jin Tonghui, Peydayesh Mohammad, Mezzenga Raffaele
ETH Zurich, Department of Health Sciences and Technology, 8092 Zurich, Switzerland.
ETH Zurich, Department of Health Sciences and Technology, 8092 Zurich, Switzerland; ETH Zurich, Department of Materials, Wolfgang-Pauli-Strasse 10, 8093 Zurich, Switzerland.
Environ Int. 2021 Dec;157:106876. doi: 10.1016/j.envint.2021.106876. Epub 2021 Sep 14.
Water purification from per- and poly-fluoroalkyl substances (PFASs), as a group of persistent and mobile fluoro-organic contaminants, is receiving increasing attention worldwide due to the ubiquitous presence of these highly toxic compounds. To reduce the risk of exposure of human life to PFASs and their dispersion in the environment, various techniques, primarily based on membrane technologies, have been rapidly developed. Here we critically review and analyze the current state-of-the-art of membrane-based techniques for PFASs removal, including direct membrane filtrations, adsorption-based membranes, and hybrid membrane processes. Membranes performance, treatment efficiencies, characteristic parameters and mechanisms for PFASs removal are discussed in detail. We highlight and discuss advantages and limitations, as well as challenges and prospects of individual membrane-based PFASs treatments, pointing towards the practical and sustainable application of these technologies.
从全氟和多氟烷基物质(PFASs)中净化水,作为一类持久性和流动性的氟有机污染物,由于这些剧毒化合物的广泛存在,正在受到全球越来越多的关注。为了降低人类生命接触PFASs及其在环境中扩散的风险,主要基于膜技术的各种技术已迅速发展。在此,我们对用于去除PFASs的膜基技术的当前技术水平进行了批判性回顾和分析,包括直接膜过滤、基于吸附的膜和混合膜工艺。详细讨论了膜的性能、处理效率、特征参数以及去除PFASs的机制。我们重点讨论了基于膜的PFASs单独处理的优点和局限性,以及挑战和前景,指出了这些技术的实际和可持续应用方向。