Department of Physics, University of California, Santa Cruz, California 95064, United States.
Department of Physics, University of California, Berkeley, California 94720, United States.
Nano Lett. 2021 Nov 10;21(21):8993-8998. doi: 10.1021/acs.nanolett.1c02271. Epub 2021 Oct 26.
Experimental realizations of graphene-based stadium-shaped quantum dots (QDs) have been few and have been incompatible with scanned probe microscopy. Yet, the direct visualization of electronic states within these QDs is crucial for determining the existence of quantum chaos in these systems. We report the fabrication and characterization of electrostatically defined stadium-shaped QDs in heterostructure devices composed of monolayer graphene (MLG) and bilayer graphene (BLG). To realize a stadium-shaped QD, we utilized the tip of a scanning tunneling microscope to charge defects in a supporting hexagonal boron nitride flake. The stadium states visualized are consistent with tight-binding-based simulations but lack clear quantum chaos signatures. The absence of quantum chaos features in MLG-based stadium QDs is attributed to the leaky nature of the confinement potential due to Klein tunneling. In contrast, for BLG-based stadium QDs (which have stronger confinement) quantum chaos is precluded by the smooth confinement potential which reduces interference and mixing between states.
基于石墨烯的体育场形量子点(QD)的实验实现很少,并且与扫描探针显微镜不兼容。然而,直接观察这些 QD 中的电子态对于确定这些系统中量子混沌的存在至关重要。我们报告了由单层石墨烯(MLG)和双层石墨烯(BLG)组成的异质结构器件中静电定义的体育场形 QD 的制造和特性。为了实现体育场形 QD,我们利用扫描隧道显微镜的尖端在支撑的六方氮化硼薄片中对缺陷进行充电。可视化的体育场态与基于紧束缚的模拟一致,但缺乏明显的量子混沌特征。由于 Klein 隧道,MLG 基体育场 QD 中不存在量子混沌特征归因于限制势的泄漏性质。相比之下,对于基于 BLG 的体育场 QD(具有更强的限制),由于限制势平滑,减少了状态之间的干扰和混合,从而排除了量子混沌。