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基于无机钙钛矿CsPbBr₃/GeSn异质结的宽带光电探测器

Broadband Photodetector Based on Inorganic Perovskite CsPbBr /GeSn Heterojunction.

作者信息

Cong Hui, Chu Xinbo, Wan Fengshuo, Chu Zema, Wang Xiaoyu, Ma Yao, Jiang Jizhong, Shen Liang, You Jingbi, Xue Chunlai

机构信息

State Key Laboratory for Supperlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Science, Beijing, 100083, P. R. China.

Key Laboratory of Semiconductor Materials Science, Institute of Semiconductors, Chinese Academy of Science, Beijing, 100083, P. R. China.

出版信息

Small Methods. 2021 Aug;5(8):e2100517. doi: 10.1002/smtd.202100517. Epub 2021 Jun 23.

Abstract

Photodetectors with broadband response spectrum have attracted great interest in many application areas such as imaging, gas sensing, and night vision. Here, a high performance broadband photodetector is demonstrated with inorganic perovskite CsPbBr /GeSn heterojunction, detection range can be covered from 450 to 2200 nm. The responsivity of heterojunction device can achieve as high as 129 mA W under illuminated light of 532 nm, which is 4.92 times larger than that of a GeSn based device. As the CsPbBr can also act as anti-reflective coating for infrared wavelength, the infrared band responsivity at wavelength of 2200 nm can also be raised by 1.42 times. In addition, the device with all inorganic components is showed good stability, while keeping in the dry environment, the device can sustain its 90% original after 550 h storage. These results show the inorganic perovskite/GeSn heterojunction device is of great potential in broadband photodetection with high responsivity.

摘要

具有宽带响应光谱的光电探测器在成像、气体传感和夜视等许多应用领域引起了极大的关注。在此,展示了一种高性能宽带光电探测器,其采用无机钙钛矿CsPbBr/GeSn异质结,检测范围可覆盖450至2200纳米。在532纳米的光照下,异质结器件的响应度可高达129毫安/瓦,比基于GeSn的器件大4.92倍。由于CsPbBr还可作为红外波长的抗反射涂层,2200纳米波长处的红外波段响应度也可提高1.42倍。此外,具有全无机成分的器件表现出良好的稳定性,在干燥环境中保存550小时后,器件仍可保持其原始性能的90%。这些结果表明,无机钙钛矿/GeSn异质结器件在高响应度宽带光电探测方面具有巨大潜力。

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