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基于Si /Ni自掺杂NiO钝化接触的具有增强功率转换效率的异质结构硅太阳能电池。

Heterostructure Silicon Solar Cells with Enhanced Power Conversion Efficiency Based on Si /Ni Self-Doped NiO Passivating Contact.

作者信息

Zhang Wei, Shen Honglie, Yin Min, Lu Linfeng, Xu Binbin, Li Dongdong

机构信息

College of Science, Jiangsu Key Laboratory of Materials and Technology for Energy Conversion, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, PR China.

The Interdisciplinary Research Center, Shanghai Advanced Research Institute, Chinese Academy of Sciences, 99 Haike Road, Zhangjiang Hi-Tech Park, Pudong, Shanghai 201210, China.

出版信息

ACS Omega. 2022 May 5;7(19):16494-16501. doi: 10.1021/acsomega.2c00496. eCollection 2022 May 17.

DOI:10.1021/acsomega.2c00496
PMID:35601318
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9118205/
Abstract

Developing efficient crystalline silicon/wide-band gap metal-oxide thin-film heterostructure junction-based crystalline silicon (-Si) solar cells has been an attractive alternative to the silicon thin film-based counterparts. Herein, nickel oxide thin films are introduced as the hole-selective layer for -Si solar cells and prepared using the reactive sputtering technique with the target of metallic nickel. An optimal Ni self-doped NiO film is obtained by tuning the reactive oxygen atmosphere to construct the optimized -Si/NiO heterostructure band alignment. A thin SiO interlayer was further introduced to reduce the defect of the -Si/NiO interface with the UV-ozone (UVO) treatment. The constructed -type -Si/SiO /NiO /Ag solar cell exhibits an increase in the open voltage from 586 to 611 mV and achieves a 19.2% conversion efficiency.

摘要

开发高效的基于晶体硅/宽带隙金属氧化物薄膜异质结构结的晶体硅（c-Si）太阳能电池，一直是基于硅薄膜的同类电池颇具吸引力的替代方案。在此，氧化镍薄膜被引入作为c-Si太阳能电池的空穴选择性层，并采用以金属镍为靶材的反应溅射技术制备。通过调节反应性氧气氛以构建优化的c-Si/NiO异质结构能带排列，获得了最佳的Ni自掺杂NiO薄膜。进一步引入薄的SiO₂ 中间层，通过紫外臭氧（UVO）处理来减少c-Si/NiO界面的缺陷。所构建的p型c-Si/SiO₂ /NiO/Ag太阳能电池的开路电压从586 mV提高到611 mV，实现了19.2%的转换效率。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/6df68a5139bd/ao2c00496_0008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/5a86983c2131/ao2c00496_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/b82038ce17c8/ao2c00496_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/4477bee5a87c/ao2c00496_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/ef34d255aa5f/ao2c00496_0005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/219f70d8d7f3/ao2c00496_0006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/19279e7cf215/ao2c00496_0007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/6df68a5139bd/ao2c00496_0008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/5a86983c2131/ao2c00496_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/b82038ce17c8/ao2c00496_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/4477bee5a87c/ao2c00496_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/ef34d255aa5f/ao2c00496_0005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/219f70d8d7f3/ao2c00496_0006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/19279e7cf215/ao2c00496_0007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/1a41/9118205/6df68a5139bd/ao2c00496_0008.jpg

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