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在磁握手材料中进行编程交互。

Programming interactions in magnetic handshake materials.

机构信息

School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, 02139, USA.

School of Applied and Engineering Physics, Cornell University, Ithaca, NY, 14853, USA.

出版信息

Soft Matter. 2022 Aug 31;18(34):6404-6410. doi: 10.1039/d2sm00604a.

Abstract

The ability to rapidly manufacture building blocks with specific binding interactions is a key aspect of programmable assembly. Recent developments in DNA nanotechnology and colloidal particle synthesis have significantly advanced our ability to create particle sets with programmable interactions, based on DNA or shape complementarity. The increasing miniaturization underlying magnetic storage offers a new path for engineering programmable components for self assembly, by printing magnetic dipole patterns on substrates using nanotechnology. How to efficiently design dipole patterns for programmable assembly remains an open question as the design space is combinatorially large. Here, we present design rules for programming these magnetic interactions. By optimizing the structure of the dipole pattern, we demonstrate that the number of independent building blocks scales super linearly with the number of printed domains. We test these design rules using computational simulations of self assembled blocks, and experimental realizations of the blocks at the mm scale, demonstrating that the designed blocks give high yield assembly. In addition, our design rules indicate that with current printing technology, micron sized magnetic panels could easily achieve hundreds of different building blocks.

摘要

快速制造具有特定结合相互作用的构建块的能力是可编程组装的一个关键方面。最近在 DNA 纳米技术和胶体粒子合成方面的发展极大地提高了我们基于 DNA 或形状互补性创建具有可编程相互作用的粒子集的能力。磁存储的不断小型化为自组装工程可编程组件提供了一条新途径,通过使用纳米技术在基板上打印磁偶极子图案。由于设计空间组合庞大,如何有效地为可编程组装设计偶极子图案仍然是一个悬而未决的问题。在这里,我们提出了用于编程这些磁相互作用的设计规则。通过优化偶极子图案的结构,我们证明了独立构建块的数量与打印域的数量呈超线性比例缩放。我们使用自组装块的计算模拟和毫米级实验实现来测试这些设计规则,证明了所设计的块具有高产量的组装。此外,我们的设计规则表明,使用当前的打印技术,微米大小的磁性面板可以轻松实现数百种不同的构建块。

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