Department of Electrical Engineering and Computer Science, University of Michigan, 1301 Beal Avenue, Ann Arbor, Michigan48109, United States.
Department of Materials Science and Engineering, University of Michigan, 2300 Hayward Street, Ann Arbor, Michigan48109, United States.
Nano Lett. 2023 Mar 8;23(5):1680-1687. doi: 10.1021/acs.nanolett.2c04220. Epub 2023 Feb 2.
High efficiency micro-LEDs, with lateral dimensions as small as one micrometer, are desired for next-generation displays, virtual/augmented reality, and ultrahigh-speed optical interconnects. The efficiency of quantum well LEDs, however, is reduced to negligibly small values when scaled to such small dimensions. Here, we show such a fundamental challenge can be overcome by developing nanowire excitonic LEDs. Harnessing the large exciton oscillator strength of quantum-confined nanostructures, we demonstrate a submicron scale green-emitting LED having an external quantum efficiency and wall-plug efficiency of 25.2% and 20.7%, respectively, the highest values reported for any LEDs of this size to our knowledge. We established critical factors for achieving excitonic micro-LEDs, including the epitaxy of nanostructures to achieve strain relaxation, the utilization of semipolar planes to minimize polarization effects, and the formation of nanoscale quantum-confinement to enhance electron-hole wave function overlap. This work provides a viable path to break the efficiency bottleneck of nanoscale optoelectronics.
高效率微发光二极管(micro-LED)的尺寸可达一微米,是下一代显示器、虚拟现实/增强现实和超高速度光互连的理想选择。然而,当尺寸缩小到如此小的尺寸时,量子阱 LED 的效率会降低到可以忽略不计的值。在这里,我们通过开发纳米线激子 LED 来克服这一基本挑战。利用量子限制纳米结构的大激子振荡器强度,我们展示了一个亚微米级的绿色发光 LED,其外量子效率和功率转换效率分别为 25.2%和 20.7%,据我们所知,这是此类尺寸的 LED 中报道的最高值。我们确定了实现激子微 LED 的关键因素,包括实现应变弛豫的纳米结构外延、利用半极性平面最小化极化效应以及形成纳米级量子限制以增强电子-空穴波函数重叠。这项工作为突破纳米光电学的效率瓶颈提供了可行的途径。