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中心对称范德瓦尔斯铁锗碲中梅尔ons 与斯格明子共存。

Coexistence of Merons with Skyrmions in the Centrosymmetric Van Der Waals Ferromagnet Fe GeTe.

机构信息

National High Magnetic Field Laboratory, Tallahassee, FL, 32310, USA.

Materials Science Division, Argonne National Laboratory, Lemont, IL, 60439, USA.

出版信息

Adv Mater. 2023 Apr;35(17):e2212087. doi: 10.1002/adma.202212087. Epub 2023 Mar 16.

Abstract

Fe GeTe is a centrosymmetric, layered van der Waals (vdW) ferromagnet that displays Curie temperatures T (270-330 K) that are within the useful range for spintronic applications. However, little is known about the interplay between its topological spin textures (e.g., merons, skyrmions) with technologically relevant transport properties such as the topological Hall effect (THE) or topological thermal transport. Here, via high-resolution Lorentz transmission electron microscopy, it is shown that merons and anti-meron pairs coexist with Néel skyrmions in Fe GeTe over a wide range of temperatures and probe their effects on thermal and electrical transport. A THE is detected, even at room T, that senses merons at higher T's, as well as their coexistence with skyrmions as T is lowered, indicating an on-demand thermally driven formation of either type of spin texture. Remarkably, an unconventional THE is also observed in absence of Lorentz force, and it is attributed to the interaction between charge carriers and magnetic field-induced chiral spin textures. These results expose Fe GeTe as a promising candidate for the development of applications in skyrmionics/meronics due to the interplay between distinct but coexisting topological magnetic textures and unconventional transport of charge/heat carriers.

摘要

FeGeTe 是一种中心对称的层状范德华(vdW)铁磁体,其居里温度 T(270-330K)在用于自旋电子学应用的有用范围内。然而,对于其拓扑自旋织构(例如,梅尔恩斯,斯格明子)与技术相关的传输特性(例如拓扑霍尔效应(THE)或拓扑热传输)之间的相互作用知之甚少。在这里,通过高分辨率的洛伦兹透射电子显微镜,发现在 FeGeTe 中,梅尔恩斯和反梅尔恩斯对与奈尔斯格明子在很宽的温度范围内共存,并探测它们对热和电输运的影响。即使在室温 T 下,也检测到了 THE,它可以感应到更高温度下的梅尔恩斯,以及随着温度降低与斯格明子共存,表明这两种类型的自旋织构可以按需热驱动形成。值得注意的是,在没有洛伦兹力的情况下也观察到了非传统的 THE,这归因于载流子与磁场诱导的手征自旋织构之间的相互作用。这些结果表明,由于不同但共存的拓扑磁织构和电荷/热载流子的非传统输运之间的相互作用,FeGeTe 是发展斯格明子/梅尔恩斯应用的有前途的候选材料。

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