RIKEN Center for Emergent Matter Science, Wako-shi, Saitama 351-0198, Japan.
Physics & Informatics Laboratories (PHI Lab), NTT Research, Inc., Sunnyvale, California 94085, United States.
Nano Lett. 2023 May 24;23(10):4564-4571. doi: 10.1021/acs.nanolett.3c01021. Epub 2023 May 2.
The rotational response of quantum condensed fluids is strikingly distinct from rotating classical fluids, especially notable for the excitation and ordering of quantized vortex ensembles. Although widely studied in conservative systems, the dynamics of rotating open-dissipative superfluids such as exciton-polariton condensates remains largely unexplored, as it requires high-frequency rotation while avoiding resonantly driving the condensate. We create a rotating polariton condensate at gigahertz frequencies by off-resonantly pumping with a rotating optical stirrer composed of the time-dependent interference of two frequency-offset, structured laser modes. Acquisition of angular momentum exceeding the critical 1/particle is directly measured, accompanied by the deterministic nucleation and capture of quantized vortices with a handedness controlled by the pump rotation direction. The demonstration of controlled optical rotation of a spontaneously formed polariton condensate enables new opportunities for the study of open dissipative superfluidity, ordering of non-Hermitian quantized vortex matter, and topological states in a highly nonlinear, photonic platform.
量子凝聚态流体的旋转响应与旋转经典流体明显不同,特别是在激发和有序量子涡旋集合方面。尽管在保守系统中得到了广泛研究,但旋转开放耗散超流体(如激子极化激元凝聚体)的动力学仍然在很大程度上未被探索,因为它需要高频旋转,同时避免共振驱动凝聚体。我们通过使用由两个频移、结构化激光模式的时变干涉组成的旋转光学搅拌器,在千兆赫兹频率下产生旋转极化激元凝聚体。直接测量到超过临界 1/粒子的角动量获取,伴随着由泵旋转方向控制的手性的量子涡旋的确定性成核和捕获。自发形成的极化激元凝聚体的受控光学旋转的演示为研究开放耗散超流性、非厄米量子涡旋物质的有序性以及高度非线性光子平台中的拓扑状态提供了新的机会。