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对从垃圾渗滤液中去除全氟和多氟烷基物质 (PFAS) 的发生、监测和去除技术的综述。

A review of the occurrence, monitoring, and removal technologies for the remediation of per- and polyfluoroalkyl substances (PFAS) from landfill leachate.

机构信息

College of Science and Technology, Hebei Agricultural University, Cangzhou, 061100, China; Key Laboratory of Water Cycle and Related Land Surface Processes, Institute of Geographic Science and Natural Resources Research, Chinese Academy of Science, Beijing, 100101, China.

Key Laboratory of Water Cycle and Related Land Surface Processes, Institute of Geographic Science and Natural Resources Research, Chinese Academy of Science, Beijing, 100101, China.

出版信息

Chemosphere. 2023 Aug;332:138824. doi: 10.1016/j.chemosphere.2023.138824. Epub 2023 May 8.

Abstract

Per- and polyfluoroalkyl substances (PFAS) are persistent organic pollutants (POPs) that pose significant environmental and human health risks. The presence of PFAS in landfill leachate is becoming an increasingly concerning issue. This article presents a comprehensive review of current knowledge and research gaps in monitoring and removing PFAS from landfill leachate. The focus is on evaluating the effectiveness and sustainability of existing removal technologies, and identifying areas where further research is needed. To achieve this goal, the paper examines the existing technologies for monitoring and treating PFAS in landfill leachate. The review emphasizes the importance of sample preparation techniques and quality assurance/quality control measures in ensuring accurate and reliable results. Then, this paper reviewed the existing technologies for removal and remediation of PFAS in landfill leachates, such as adsorption, membrane filtration, photocatalytic oxidation, electrocatalysis, biodegradation, and constructed wetlands. Additionally, the paper summarizes the factors that exhibit the performance of various treatment technologies: reaction time, experimental conditions, and removal rates. Furthermore, the paper evaluates the potential application of different remediation technologies (i.e., adsorption, membrane filtration, photocatalytic oxidation, electrocatalysis, biodegradation, and constructed wetlands, etc.) in treating landfill leachate containing PFAS and its precursors, such as fluorotelomeres like FTOH and FTSs. The review highlights the importance of considering economic, technical, and environmental factors when selecting control measures. Overall, this article aims to provide guidance for promoting environmental protection and sustainable development in the context of PFAS contamination in landfill leachate.

摘要

全氟和多氟烷基物质(PFAS)是持久性有机污染物(POPs),对环境和人类健康构成重大风险。PFAS 在垃圾渗滤液中的存在正成为一个日益令人担忧的问题。本文全面回顾了监测和从垃圾渗滤液中去除 PFAS 的现有知识和研究空白。重点评估了现有去除技术的有效性和可持续性,并确定了需要进一步研究的领域。为了实现这一目标,本文检查了监测和处理垃圾渗滤液中 PFAS 的现有技术。综述强调了样品制备技术和质量保证/质量控制措施在确保准确可靠结果方面的重要性。然后,本文回顾了用于去除和修复垃圾渗滤液中 PFAS 的现有技术,如吸附、膜过滤、光催化氧化、电催化、生物降解和人工湿地。此外,本文总结了各种处理技术的性能表现因素:反应时间、实验条件和去除率。此外,本文评估了不同修复技术(如吸附、膜过滤、光催化氧化、电催化、生物降解和人工湿地等)在处理含有 PFAS 及其前体(如 FTOH 和 FTS 等氟代烯烃)的垃圾渗滤液方面的潜在应用。综述强调了在选择控制措施时考虑经济、技术和环境因素的重要性。总体而言,本文旨在为在 PFAS 污染的背景下促进环境保护和可持续发展提供指导。

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