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由于带隙梯级态的量子雪崩导致关联绝缘子崩塌。

Correlated insulator collapse due to quantum avalanche via in-gap ladder states.

机构信息

Department of Physics, State University of New York at Buffalo, Buffalo, NY, 14260, USA.

Laboratoire de Physique de l'École Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université Paris Cité, F-75005, Paris, France.

出版信息

Nat Commun. 2023 May 22;14(1):2936. doi: 10.1038/s41467-023-38557-8.

Abstract

The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche.

摘要

在远非平衡的直流电场下,关联绝缘体中的预测和实验转换场之间存在显著差异,这需要重新评估当前的微观理解。在这里,我们通过引入一个电子与声子非弹性介质耦合的通用模型,表明在这种绝缘体的体极限中,即使在任意小的电场下,也可能发生电子雪崩。通过多声子发射过程产生的带隙中的级联状态的产生,导致了量子雪崩。在雪崩中产生的热声子会引发相关能隙的过早和部分崩塌。声子谱决定了存在两阶段还是单阶段的转换事件,我们分别将其与电荷密度波和莫特电阻相变相关联。电子和声子温度的行为以及阈值场的温度依赖性表明,在量子雪崩的统一框架内,如何出现热和量子转换场景之间的交叉。

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