Department of Physics, State University of New York at Buffalo, Buffalo, NY, 14260, USA.
Laboratoire de Physique de l'École Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université Paris Cité, F-75005, Paris, France.
Nat Commun. 2023 May 22;14(1):2936. doi: 10.1038/s41467-023-38557-8.
The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche.
在远非平衡的直流电场下,关联绝缘体中的预测和实验转换场之间存在显著差异,这需要重新评估当前的微观理解。在这里,我们通过引入一个电子与声子非弹性介质耦合的通用模型,表明在这种绝缘体的体极限中,即使在任意小的电场下,也可能发生电子雪崩。通过多声子发射过程产生的带隙中的级联状态的产生,导致了量子雪崩。在雪崩中产生的热声子会引发相关能隙的过早和部分崩塌。声子谱决定了存在两阶段还是单阶段的转换事件,我们分别将其与电荷密度波和莫特电阻相变相关联。电子和声子温度的行为以及阈值场的温度依赖性表明,在量子雪崩的统一框架内,如何出现热和量子转换场景之间的交叉。