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道路、路边植被和邻近土壤中可溶性和颗粒性放射性污染物二次传输预防技术综述。

Review of technologies for preventing secondary transport of soluble and particulate radiological contamination from roadways, roadside vegetation, and adjacent soils.

作者信息

Saito Hiroshi, Sutton Mark, Zhao Pihong, Lee Sang Don, Magnuson Matthew

机构信息

Lawrence Livermore National Laboratory, P.O. Box 808, Livermore, CA 94551, United States.

US Environmental Protection Agency, Office of Research and Development, Cincinnati, OH 45268, United States.

出版信息

Environ Adv. 2020 Sep;1:1-13. doi: 10.1016/j.envadv.2020.100003.

DOI:10.1016/j.envadv.2020.100003
PMID:37229463
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10208302/
Abstract

Transport of contaminants from roadways to the environment is well known, although studies of technologies for preventing and managing this appear infrequently in the literature. This paper reviews technologies studied for radiological contaminants. In addition to nuclear facility decommissioning, nuclear power plant accidents at Chernobyl (Former Soviet Union), Fukushima (Japan) and elsewhere have provided real world situations to both develop and test technologies to remediate radiological contamination and to return roadways, along with adjacent vegetation and soil, to prior use. From publications arising from these efforts, technologies were reviewed for radioactive material with two distinct properties (water-soluble and insoluble radioactive contaminants). The reported characteristics and capabilities of technologies are summarized in this review. This review also presents logistical considerations of implementation of the technologies, including waste management which can be an extreme impediment to rapid remediation if generated quantities of hazardous waste exceed local handling capacity. The summarized literature review suggests future avenues of work, chiefly for insoluble particulates, focused on technologies which may be mechanistically applicable to their remediation. While the underlying chemical and physical mechanisms that contribute to transport differ among contaminants, the studies reviewed here might also be applicable to non-radioactive contaminants, because the presence of radioactivity is largely independent of the underlying mechanisms.

摘要

污染物从道路向环境的传输是众所周知的,尽管关于预防和管理此类传输技术的研究在文献中并不常见。本文综述了针对放射性污染物所研究的技术。除了核设施退役外,切尔诺贝利(前苏联)、福岛(日本)及其他地方的核电站事故提供了实际案例,用于开发和测试修复放射性污染以及使道路及其周边植被和土壤恢复先前用途的技术。基于这些工作产生的出版物,对具有两种不同特性(水溶性和不溶性放射性污染物)的放射性物质的技术进行了综述。本综述总结了所报道技术的特性和能力。本综述还介绍了技术实施过程中的后勤考虑因素,包括废物管理,如果危险废物产生量超过当地处理能力,这可能成为快速修复的极大障碍。综述文献表明了未来的工作方向,主要针对不溶性颗粒物,重点关注可能在机理上适用于其修复的技术。虽然不同污染物导致传输的潜在化学和物理机制有所不同,但此处综述的研究可能也适用于非放射性污染物,因为放射性的存在在很大程度上与潜在机制无关。

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本文引用的文献

1
Novel Method of Quantifying Radioactive Cesium-Rich Microparticles (CsMPs) in the Environment from the Fukushima Daiichi Nuclear Power Plant.从福岛第一核电站环境中定量放射性铯丰富的微颗粒(CsMPs)的新方法。
Environ Sci Technol. 2018 Jun 5;52(11):6390-6398. doi: 10.1021/acs.est.7b06693. Epub 2018 May 21.
2
Uranium Dioxides and Debris Fragments Released to the Environment with Cesium-Rich Microparticles from the Fukushima Daiichi Nuclear Power Plant.福岛第一核电站富铯微颗粒向环境中释放的二氧化铀和碎片。
Environ Sci Technol. 2018 Mar 6;52(5):2586-2594. doi: 10.1021/acs.est.7b06309. Epub 2018 Feb 13.
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Isotopic signature and nano-texture of cesium-rich micro-particles: Release of uranium and fission products from the Fukushima Daiichi Nuclear Power Plant.富铯微颗粒的同位素特征和纳米结构:福岛第一核电站铀和裂变产物的释放。
Sci Rep. 2017 Jul 14;7(1):5409. doi: 10.1038/s41598-017-05910-z.
4
Caesium-rich micro-particles: A window into the meltdown events at the Fukushima Daiichi Nuclear Power Plant.富含铯的微颗粒:福岛第一核电站堆芯熔毁事件的一扇窗口。
Sci Rep. 2017 Feb 15;7:42731. doi: 10.1038/srep42731.
5
Wide-area decontamination in an urban environment after radiological dispersion: A review and perspectives.城市环境中放射性物质弥散后的大面积去污:综述与展望。
J Hazard Mater. 2016 Mar 15;305:67-86. doi: 10.1016/j.jhazmat.2015.11.014. Epub 2015 Nov 18.
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Metals in European roadside soils and soil solution--a review.欧洲道路边土壤和土壤溶液中的金属元素——综述。
Environ Pollut. 2014 Jun;189:98-110. doi: 10.1016/j.envpol.2014.02.025. Epub 2014 Mar 19.
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Fukushima remediation: status and overview of future plans.福岛修复:现状和未来计划概述。
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