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用于固态染料敏化太阳能电池的光敏剂分子工程：最新进展与展望

Molecular Engineering of Photosensitizers for Solid-State Dye-Sensitized Solar Cells: Recent Developments and Perspectives.

作者信息

Yadagiri Bommaramoni, Kumar Kaliamurthy Ashok, Yoo Kicheon, Cheol Kang Hyeong, Ryu Junyeong, Kwaku Asiam Francis, Lee Jae-Joon

机构信息

Research Center for Photoenergy Harvesting and Conversion Technology (phct), Department of Energy Materials and Engineering, Dongguk University, Seoul, 04620, Republic of Korea.

出版信息

ChemistryOpen. 2023 Dec;12(12):e202300170. doi: 10.1002/open.202300170. Epub 2023 Oct 24.

DOI:10.1002/open.202300170
PMID:37874016
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10695739/
Abstract

Dye-sensitized solar cells (DSSCs) are a feasible alternative to traditional silicon-based solar cells because of their low cost, eco-friendliness, flexibility, and acceptable device efficiency. In recent years, solid-state DSSCs (ss-DSSCs) have garnered much interest as they can overcome the leakage and evaporation issues of liquid electrolyte systems. However, the poor morphology of solid electrolytes and their interface with photoanodes can minimize the device performance. The photosensitizer/dye is a critical component of ss-DSSCs and plays a vital role in the device's overall performance. In this review, we summarize recent developments and performance of photosensitizers, including mono- and co-sensitization of ruthenium, porphyrin, and metal-free organic dyes under 1 sun and ambient/artificial light conditions. We also discuss the various requirements that efficient photosensitizers should satisfy and provide an overview of their historical development over the years.

摘要

染料敏化太阳能电池（DSSC）因其低成本、环保、柔韧性以及可接受的器件效率，成为传统硅基太阳能电池的一种可行替代方案。近年来，固态染料敏化太阳能电池（ss-DSSC）备受关注，因为它们能够克服液体电解质系统的泄漏和蒸发问题。然而，固体电解质及其与光阳极的界面形态不佳会降低器件性能。光敏剂/染料是ss-DSSC的关键组件，对器件的整体性能起着至关重要的作用。在本综述中，我们总结了光敏剂的最新进展和性能，包括钌、卟啉和无金属有机染料在1个太阳光照以及环境光/人造光条件下的单敏化和共敏化。我们还讨论了高效光敏剂应满足的各种要求，并概述了它们多年来的历史发展。

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