Bitenc Jan, Pirnat Klemen, Lužanin Olivera, Dominko Robert
National Institute of Chemistry, Hajdrihova 19, 1000 Ljubljana, Slovenia.
Faculty of Chemistry and Chemical Technology, University of Ljubljana, Večna pot 113, 1000 Ljubljana, Slovenia.
Chem Mater. 2024 Jan 16;36(3):1025-1040. doi: 10.1021/acs.chemmater.3c02408. eCollection 2024 Feb 13.
Organic active materials are seen as next-generation battery materials that could circumvent the sustainability and cost limitations connected with the current Li-ion battery technology while at the same time enabling novel battery functionalities like a bioderived feedstock, biodegradability, and mechanical flexibility. Many promising research results have recently been published. However, the reproducibility and comparison of the literature results are somehow limited due to highly variable electrode formulations and electrochemical testing conditions. In this Perspective, we provide a critical view of the organic cathode active materials and suggest future guidelines for electrochemical characterization, capacity evaluation, and mechanistic investigation to facilitate reproducibility and benchmarking of literature results, leading to the accelerated development of organic electrode active materials for practical applications.
有机活性材料被视为下一代电池材料,它可以规避与当前锂离子电池技术相关的可持续性和成本限制,同时实现新型电池功能,如生物衍生原料、生物可降解性和机械柔韧性。最近已经发表了许多有前景的研究成果。然而,由于电极配方和电化学测试条件高度可变,文献结果的可重复性和可比性在一定程度上受到限制。在这篇观点文章中,我们对有机阴极活性材料进行了批判性审视,并提出了未来电化学表征、容量评估和机理研究的指导方针,以促进文献结果的可重复性和基准测试,从而加速有机电极活性材料在实际应用中的开发。