Department of Mechanical Engineering, University of California at Berkeley, Berkeley, CA, USA.
Department of Mechanical Engineering, University of Utah, Salt Lake City, UT, USA.
Nature. 2024 May;629(8010):67-73. doi: 10.1038/s41586-024-07279-2. Epub 2024 Apr 17.
It is well established that near-field radiative heat transfer (NFRHT) can exceed Planck's blackbody limit by orders of magnitude owing to the tunnelling of evanescent electromagnetic frustrated and surface modes, as has been demonstrated experimentally for NFRHT between two large parallel surfaces and between two subwavelength membranes. However, although nanostructures can also sustain a much richer variety of localized electromagnetic modes at their corners and edges, the contributions of such additional modes to further enhancing NFRHT remain unexplored. Here we demonstrate both theoretically and experimentally a physical mechanism of NFRHT mediated by the corner and edge modes, and show that it can dominate the NFRHT in the 'dual nanoscale regime' in which both the thickness of the emitter and receiver, and their gap spacing, are much smaller than the thermal photon wavelengths. For two coplanar 20-nm-thick silicon carbide membranes separated by a 100-nm vacuum gap, the NFRHT coefficient at room temperature is both predicted and measured to be 830 W m K, which is 5.5 times larger than that for two infinite silicon carbide surfaces separated by the same gap, and 1,400 times larger than the corresponding blackbody limit accounting for the geometric view factor between two coplanar membranes. This enhancement is dominated by the electromagnetic corner and edge modes, which account for 81% of the NFRHT between the silicon carbide membranes. These findings are important for future NFRHT applications in thermal management and energy conversion.
众所周知,由于渐逝电磁受挫和表面模式的隧道效应,近场辐射热传递(NFRHT)可以超过普朗克黑体极限几个数量级,这已经通过两个大平行表面和两个亚波长膜之间的 NFRHT 实验得到证实。然而,尽管纳米结构在其角落和边缘处也能维持更丰富的局域电磁模式,但这些额外模式对进一步增强 NFRHT 的贡献仍未得到探索。在这里,我们从理论和实验上证明了由角和边缘模式介导的 NFRHT 的物理机制,并表明它可以在“双纳米尺度”中主导 NFRHT,在这种情况下,发射器和接收器的厚度以及它们的间隙间隔都远小于热光子波长。对于两个由 100nm 真空间隙隔开的共面 20nm 厚碳化硅膜,在室温下,NFRHT 系数被预测和测量为 830W m K,这比两个具有相同间隙的无限大碳化硅表面之间的 NFRHT 系数大 5.5 倍,比考虑到两个共面膜之间的几何视角因子的相应黑体极限大 1400 倍。这种增强主要由电磁角和边缘模式主导,它们占碳化硅膜之间 NFRHT 的 81%。这些发现对未来在热管理和能量转换中应用 NFRHT 具有重要意义。