• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

快速压缩拉曼显微光谱法用于对天然海洋环境中的微塑料进行成像和分类。

Fast compressive Raman micro-spectroscopy to image and classify microplastics from natural marine environment.

作者信息

Grand Clément, Scotté Camille, Prado Énora, El Rakwe Maria, Fauvarque Olivier, Rigneault Hervé

机构信息

Aix Marseille Univ, CNRS, Centrale Med, Institut Fresnel, Marseille, France.

INRAE, UMR ITAP, 361 Rue Jean François Breton, Montpellier 34090, France.

出版信息

Environ Technol Innov. 2024 May;34:103622. doi: 10.1016/j.eti.2024.103622.

DOI:10.1016/j.eti.2024.103622
PMID:38706940
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11066848/
Abstract

The fast and reliable detection of micron-sized plastic particles from the natural marine environment is an important topic that is mostly addressed using spontaneous Raman spectroscopy. Due to the long (>tens of ms) integration time required to record a viable Raman signal, measurements are limited to a single point per microplastic particle or require very long acquisition times (up to tens of hours). In this work, we develop, validate, and demonstrate a compressive Raman technology using binary spectral filters and single-pixel detection that can image and classify six types of marine microplastic particles over an area of 1 mm with a pixel dwell time down to 1.75 ms/pixel and a spatial resolution of 1 µm. This is x10-100 faster than reported in previous studies.

摘要

从天然海洋环境中快速可靠地检测微米级塑料颗粒是一个重要课题,目前大多通过自发拉曼光谱法来解决。由于记录可用拉曼信号需要较长(>数十毫秒)的积分时间,测量仅限于每个微塑料颗粒的单个点,或者需要很长的采集时间(长达数十小时)。在这项工作中,我们开发、验证并展示了一种使用二元光谱滤波器和单像素检测的压缩拉曼技术,该技术能够在1平方毫米的区域内对六种海洋微塑料颗粒进行成像和分类,像素驻留时间低至1.75毫秒/像素,空间分辨率为1微米。这比之前研究报告的速度快10至100倍。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/e81fbd7f00c0/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/74e872c17857/ga1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/90463df13cb4/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/be2657b8379a/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/0c264b145bba/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/6d35b2639813/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/2e7244bd69ba/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/8e3f7f8e9368/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/e81fbd7f00c0/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/74e872c17857/ga1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/90463df13cb4/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/be2657b8379a/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/0c264b145bba/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/6d35b2639813/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/2e7244bd69ba/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/8e3f7f8e9368/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/205a/11066848/e81fbd7f00c0/gr7.jpg

相似文献

1
Fast compressive Raman micro-spectroscopy to image and classify microplastics from natural marine environment.快速压缩拉曼显微光谱法用于对天然海洋环境中的微塑料进行成像和分类。
Environ Technol Innov. 2024 May;34:103622. doi: 10.1016/j.eti.2024.103622.
2
Prevalence of small-sized microplastics in coastal sediments detected by multipoint confocal micro-Raman spectrum scanning.多点共焦显微拉曼光谱扫描检测沿海沉积物中小尺寸微塑料的流行率。
Sci Total Environ. 2022 Jul 20;831:154741. doi: 10.1016/j.scitotenv.2022.154741. Epub 2022 Mar 24.
3
Analysis of microplastics in water by micro-Raman spectroscopy: Release of plastic particles from different packaging into mineral water.利用微拉曼光谱分析水中的微塑料:不同包装材料向矿泉水释放塑料颗粒。
Water Res. 2018 Feb 1;129:154-162. doi: 10.1016/j.watres.2017.11.011. Epub 2017 Nov 6.
4
Development of an optimal filter substrate for the identification of small microplastic particles in food by micro-Raman spectroscopy.开发用于通过显微拉曼光谱法识别食品中微小塑料颗粒的最佳滤膜基质。
Anal Bioanal Chem. 2017 Jun;409(16):4099-4109. doi: 10.1007/s00216-017-0358-y. Epub 2017 Apr 24.
5
Rapid identification of micro and nanoplastics by line scan Raman micro-spectroscopy.通过线扫描拉曼显微光谱快速识别微塑料和纳米塑料。
Talanta. 2024 Jan 1;266(Pt 2):125067. doi: 10.1016/j.talanta.2023.125067. Epub 2023 Aug 9.
6
Detection of microplastics based on splicing grating spatial heterodyne Raman spectroscopy.基于拼接光栅空间外差拉曼光谱的微塑料检测
Spectrochim Acta A Mol Biomol Spectrosc. 2024 Oct 5;318:124499. doi: 10.1016/j.saa.2024.124499. Epub 2024 May 22.
7
Surface-Enhanced Raman Spectroscopy Facilitates the Detection of Microplastics <1 μm in the Environment.表面增强拉曼光谱有助于检测环境中 <1 μm 的微塑料。
Environ Sci Technol. 2020 Dec 15;54(24):15594-15603. doi: 10.1021/acs.est.0c02317. Epub 2020 Oct 23.
8
Hyperspectral imaging for identification of irregular-shaped microplastics in water.用于识别水中不规则形状微塑料的高光谱成像技术。
Sci Total Environ. 2024 Sep 20;944:173811. doi: 10.1016/j.scitotenv.2024.173811. Epub 2024 Jun 8.
9
Raman imaging for the analysis of silicone microplastics and nanoplastics released from a kitchen sealant.用于分析从厨房密封剂中释放的硅基微塑料和纳米塑料的拉曼成像技术。
Front Chem. 2023 May 17;11:1165523. doi: 10.3389/fchem.2023.1165523. eCollection 2023.
10
Analysis of environmental microplastics by vibrational microspectroscopy: FTIR, Raman or both?通过振动光谱分析环境中的微塑料:傅里叶变换红外光谱、拉曼光谱还是两者兼用?
Anal Bioanal Chem. 2016 Nov;408(29):8377-8391. doi: 10.1007/s00216-016-9956-3. Epub 2016 Oct 8.

本文引用的文献

1
Fast Compressive Raman Imaging of Polymorph Molecules and Excipients in Pharmaceutical Tablets.快速压缩拉曼成像在药物片剂中多晶型分子和赋形剂的应用。
Anal Chem. 2022 Dec 6;94(48):16632-16637. doi: 10.1021/acs.analchem.2c02680. Epub 2022 Nov 23.
2
Shot-noise limited tunable dual-vibrational frequency stimulated Raman scattering microscopy.散粒噪声限制的可调谐双振动频率受激拉曼散射显微镜
Biomed Opt Express. 2021 Nov 24;12(12):7780-7789. doi: 10.1364/BOE.446348. eCollection 2021 Dec 1.
3
Development of an Easy-to-Operate Underwater Raman System for Deep-Sea Cold Seep and Hydrothermal Vent In Situ Detection.
开发一种易于操作的深海冷泉和热液喷口原位检测水下拉曼系统。
Sensors (Basel). 2021 Jul 27;21(15):5090. doi: 10.3390/s21155090.
4
Stimulated Raman microspectroscopy as a new method to classify microfibers from environmental samples.受激拉曼微光谱法作为一种从环境样本中分类微纤维的新方法。
Environ Pollut. 2020 Dec;267:115640. doi: 10.1016/j.envpol.2020.115640. Epub 2020 Sep 16.
5
Estimation of the mass of microplastics ingested - A pivotal first step towards human health risk assessment.摄入微塑料的质量估算——迈向人类健康风险评估的关键第一步。
J Hazard Mater. 2021 Feb 15;404(Pt B):124004. doi: 10.1016/j.jhazmat.2020.124004. Epub 2020 Oct 6.
6
Compressed Raman classification method with upper-bounded error probability.带误差概率上界的压缩 Raman 分类方法。
Opt Lett. 2019 Dec 1;44(23):5836-5839. doi: 10.1364/OL.44.005836.
7
Identification and visualisation of microplastics by Raman mapping.通过拉曼映射识别和可视化微塑料。
Anal Chim Acta. 2019 Oct 24;1077:191-199. doi: 10.1016/j.aca.2019.05.021. Epub 2019 May 16.
8
Bhattacharyya bound for Raman spectrum classification with a couple of binary filters.使用一对二元滤波器的拉曼光谱分类的巴塔查里亚界
Opt Lett. 2019 May 1;44(9):2228-2231. doi: 10.1364/OL.44.002228.
9
Identification of microplastics using Raman spectroscopy: Latest developments and future prospects.利用拉曼光谱识别微塑料:最新进展和未来展望。
Water Res. 2018 Oct 1;142:426-440. doi: 10.1016/j.watres.2018.05.060. Epub 2018 Jun 6.
10
Assessment of Compressive Raman versus Hyperspectral Raman for Microcalcification Chemical Imaging.微钙化化学成像中压缩拉曼与高光谱拉曼的评估。
Anal Chem. 2018 Jun 19;90(12):7197-7203. doi: 10.1021/acs.analchem.7b05303. Epub 2018 May 25.