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2015-2020 年中国小时臭氧浓度的简约估计。

Parsimonious estimation of hourly surface ozone concentration across China during 2015-2020.

机构信息

State Key Laboratory of Urban and Regional Ecology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China.

University of Chinese Academy of Sciences, Beijing, 100049, China.

出版信息

Sci Data. 2024 May 14;11(1):492. doi: 10.1038/s41597-024-03302-3.

Abstract

Surface ozone is an important air pollutant detrimental to human health and vegetation productivity, particularly in China. However, high resolution surface ozone concentration data is still lacking, largely hindering accurate assessment of associated environmental impacts. Here, we collected hourly ground ozone observations (over 6 million records), remote sensing products, meteorological data, and social-economic information, and applied recurrent neural networks to map hourly surface ozone data (HrSOD) at a 0.1° × 0.1° resolution across China during 2015-2020. The coefficient of determination (R) values in sample-based, site-based, and by-year cross-validations were 0.72, 0.65 and 0.71, respectively, with the root mean square error (RMSE) values being 11.71 ppb (mean = 30.89 ppb), 12.81 ppb (mean = 30.96 ppb) and 11.14 ppb (mean = 31.26 ppb). Moreover, it exhibits high spatiotemporal consistency with ground-level observations at different time scales (diurnal, seasonal, annual), and at various spatial levels (individual sites and regional scales). Meanwhile, the HrSOD provides critical information for fine-resolution assessment of surface ozone impacts on environmental and human benefits.

摘要

地面臭氧是一种重要的空气污染物,对人类健康和植被生产力有害,尤其是在中国。然而,高分辨率的地面臭氧浓度数据仍然缺乏,这在很大程度上阻碍了对相关环境影响的准确评估。在这里,我们收集了 2015-2020 年期间每小时的地面臭氧观测数据(超过 600 万条记录)、遥感产品、气象数据和社会经济信息,并应用递归神经网络绘制了 2015-2020 年期间中国每小时地面臭氧数据(HrSOD)的 0.1°×0.1°分辨率地图。在样本基础、站点基础和年度交叉验证中的决定系数(R)值分别为 0.72、0.65 和 0.71,均方根误差(RMSE)值分别为 11.71 ppb(平均值为 30.89 ppb)、12.81 ppb(平均值为 30.96 ppb)和 11.14 ppb(平均值为 31.26 ppb)。此外,它在不同时间尺度(日、季、年)和不同空间水平(个别站点和区域尺度)的地面观测结果具有高度的时空一致性。同时,HrSOD 为精细分辨率评估地面臭氧对环境和人类健康的影响提供了关键信息。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6560/11094007/6d298dac95d1/41597_2024_3302_Fig1_HTML.jpg

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