Straus D, Raines R, Kawashima E, Knowles J R, Gilbert W
Proc Natl Acad Sci U S A. 1985 Apr;82(8):2272-6. doi: 10.1073/pnas.82.8.2272.
We have replaced the glutamic acid-165 at the active site of chicken triosephosphate isomerase with an aspartic acid residue using site-directed mutagenesis. Expression of the mutant protein in a strain of Escherichia coli that lacks the bacterial isomerase results in a complementation phenotype that is intermediate between strains that have no isomerase and strains that produce either the wild-type chicken enzyme or the native E. coli isomerase. The value of kcat for the purified mutant enzyme when glyceraldehyde 3-phosphate is the substrate is 1/1500th that of the wild-type enzyme, and the Km is decreased by a factor of 3.6. With dihydroxyacetone phosphate as substrate, the kcat value is 1/240th that of the wild-type enzyme, and Km is 2 times higher. The value of Ki for a competitive inhibitor, phosphoglycolate, is the same for the mutant and wild-type enzymes, at 2 X 10(-5) M. By treating the enzyme-catalyzed isomerization as a simple three step process and assuming that substrate binding is diffusion limited, it is evident that the mutation of glutamic acid-165 to aspartic acid principally affects the free energy of the transition state(s) for the catalytic reaction itself.
我们利用定点诱变技术,将鸡磷酸丙糖异构酶活性位点处的谷氨酸-165替换为天冬氨酸残基。在缺乏细菌异构酶的大肠杆菌菌株中表达突变蛋白,会产生一种互补表型,该表型介于没有异构酶的菌株与产生野生型鸡酶或天然大肠杆菌异构酶的菌株之间。以3-磷酸甘油醛为底物时,纯化的突变酶的kcat值是野生型酶的1/1500,而Km降低了3.6倍。以磷酸二羟丙酮为底物时,kcat值是野生型酶的1/240,而Km高2倍。竞争性抑制剂磷酸乙醇酸的Ki值,突变酶和野生型酶相同,均为2×10(-5)M。通过将酶催化的异构化视为一个简单的三步过程,并假设底物结合受扩散限制,很明显谷氨酸-165突变为天冬氨酸主要影响催化反应本身过渡态的自由能。