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滴铸六方氮化硼纳米薄片中量子发射体产率的定量研究。

Quantitative Investigation of Quantum Emitter Yield in Drop-Casted Hexagonal Boron Nitride Nanoflakes.

作者信息

Kretzschmar Tom, Ritter Sebastian, Kumar Anand, Vogl Tobias, Eilenberger Falk, Schmidt Falko

机构信息

Institute of Applied Physics, Abbe Center of Photonics, Friedrich-Schiller-University, D-07745 Jena, Germany.

Department of Computer Engineering, School of Computation, Information and Technology, Technical University Munich, D-80333 Munich, Germany.

出版信息

ACS Appl Opt Mater. 2024 Jul 2;2(7):1427-1435. doi: 10.1021/acsaom.4c00200. eCollection 2024 Jul 26.

DOI:10.1021/acsaom.4c00200
PMID:39086657
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11287792/
Abstract

Single photon emitters (SPEs) are a key component for their use as pure photon source in quantum technologies. In this study, we investigate the generation of SPEs from drop-casted hexagonal boron nitride (hBN) nanoflakes, examining the influence of the immersion solution and the source of hBN. We show that, depending on the utilized supplier and solution, the number and quality of the emitters change. We perform a comprehensive optical characterization of the deposited nanoflakes to assess the quality of the generated SPEs. Importantly, we provide quantitative data on SPE yields, highlighting significant variations among solvents and different sources of hBN. We find that hBN from Merck drop-casted in acetone provided the best quality emitters with a < 0.1 and photoluminescence intensities above 300 kCounts/s. Their number of SPEs among all photon emitters was also the highest, with about 14%, rendering a total yield of about 1.25% of all drop-casted flakes. These numbers hold particular significance when evaluating drop-casting as a practical method for the generation of SPEs and their deposition and incorporation within existing nanophotonic systems. By choosing appropriate solvents and source materials' quality and yield of SPEs can be significantly increased, showcasing further optimization potential for the development of future quantum applications.

摘要

单光子发射器(SPEs)作为量子技术中纯光子源的关键组件。在本研究中,我们研究了从滴铸的六方氮化硼(hBN)纳米薄片中产生单光子发射器的情况,考察了浸泡溶液和hBN来源的影响。我们发现,根据所使用的供应商和溶液不同,发射器的数量和质量会发生变化。我们对沉积的纳米薄片进行了全面的光学表征,以评估所产生的单光子发射器的质量。重要的是,我们提供了单光子发射器产率的定量数据,突出了不同溶剂和不同hBN来源之间的显著差异。我们发现,默克公司的hBN滴铸在丙酮中时,能提供质量最佳的发射器,其线宽小于0.1,光致发光强度高于300 kCounts/s。在所有光子发射器中,它们的单光子发射器数量也是最高的,约为14%,占所有滴铸薄片的总产率约为1.25%。在评估滴铸作为产生单光子发射器及其在现有纳米光子系统中的沉积和整合的实用方法时,这些数据具有特别重要的意义。通过选择合适的溶剂和源材料,可以显著提高单光子发射器的质量和产率,为未来量子应用的发展展示了进一步的优化潜力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/687959e60f9a/ot4c00200_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/a626bb1ea533/ot4c00200_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/9262c4693dbd/ot4c00200_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/239e54826619/ot4c00200_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/687959e60f9a/ot4c00200_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/a626bb1ea533/ot4c00200_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/9262c4693dbd/ot4c00200_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/239e54826619/ot4c00200_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9359/11287792/687959e60f9a/ot4c00200_0004.jpg

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Nanoscale. 2024 Feb 29;16(9):4691-4702. doi: 10.1039/d3nr05305a.
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Hexagonal boron nitride exfoliation and dispersion.六方氮化硼的剥离与分散
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Organic Molecules as Origin of Visible-Range Single Photon Emission from Hexagonal Boron Nitride and Mica.有机分子是六方氮化硼和云母中可见光单光子发射的来源。
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