Liu Siyuan, Wu Yizhang, Jiang Lai, Xie Wanrong, Davis Brayden, Wang Meixiang, Zhang Lin, Liu Yihan, Xing Sicheng, Dickey Michael D, Bai Wubin
Department of Applied Physical Science, University of North Carolina at Chapel Hill, Chapel Hill, North Carolina 27514, United States.
Department of Biology, University of North Carolina, Chapel Hill, North Carolina 27514, United States.
ACS Appl Mater Interfaces. 2024 Sep 4;16(35):46538-46547. doi: 10.1021/acsami.4c10539. Epub 2024 Aug 1.
The development of wearable electronic devices for human health monitoring requires materials with high mechanical performance and sensitivity. In this study, we present a novel transparent tissue-like ionogel-based wearable sensor based on silver nanowire-reinforced ionogel nanocomposites, P(AAm--AA) ionogel-Ag NWs composite. The composite exhibits a high stretchability of 605% strain and a moderate fracture stress of about 377 kPa. The sensor also demonstrates a sensitive response to temperature changes and electrostatic adsorption. By encapsulating the nanocomposite in a polyurethane transparent film dressing, we address issues such as skin irritation and enable multidirectional stretching. Measuring resistive changes of the ionogel nanocomposite in response to corresponding strain changes enables its utility as a highly stretchable wearable sensor with excellent performance in sensitivity, stability, and repeatability. The fabricated pressure sensor array exhibits great proficiency in stress distribution, capacitance sensing, and discernment of fluctuations in both external electric fields and stress. Our findings suggest that this material holds promise for applications in wearable and flexible strain sensors, temperature sensors, pressure sensors, and actuators.
用于人体健康监测的可穿戴电子设备的发展需要具有高机械性能和灵敏度的材料。在本研究中,我们展示了一种基于银纳米线增强离子凝胶纳米复合材料(P(AAm--AA)离子凝胶-Ag NWs复合材料)的新型透明组织状离子凝胶基可穿戴传感器。该复合材料表现出605%应变的高拉伸性和约377 kPa的适度断裂应力。该传感器还对温度变化和静电吸附表现出灵敏响应。通过将纳米复合材料封装在聚氨酯透明薄膜敷料中,我们解决了诸如皮肤刺激等问题,并实现了多向拉伸。测量离子凝胶纳米复合材料响应相应应变变化的电阻变化,使其能够作为一种在灵敏度、稳定性和可重复性方面具有优异性能的高拉伸性可穿戴传感器。所制备的压力传感器阵列在应力分布、电容传感以及对外界电场和应力波动的辨别方面表现出很高的熟练度。我们的研究结果表明,这种材料在可穿戴和柔性应变传感器、温度传感器、压力传感器及致动器方面具有应用前景。