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可见光盲快速响应纳米结构SnO/Si光电探测器的光电评估

Opto-electrical evaluation of visible blind fast-response nanostructured SnO/Si photodetector.

作者信息

Salih Ethar Yahya

机构信息

College of Energy and Environmental Sciences, Al-Karkh University of Science 10081 Baghdad Iraq

出版信息

RSC Adv. 2024 Sep 2;14(38):27733-27740. doi: 10.1039/d4ra05303f. eCollection 2024 Aug 29.

DOI:10.1039/d4ra05303f
PMID:39224641
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11367619/
Abstract

In this study, a nanostructured tin(iv) oxide (SnO)/Si heterojunction UV photodetector was fabricated in response to laser pulses attained pulsed laser deposition (PLD). In particular, the photo-detection mechanisms of the proposed devices were thoroughly investigated considering multiple-profile dependency, namely, laser pulses, spectral response, and incident power. In detail, particle diameters of 25 and 41 nm with a bandgap alteration of 0.2 eV and a cut-off phenomenon at around 335 nm occurred as a result of an increase in the number of pulses from 300 to 700. The optimum photodetector (at 700 pulses, nm, and 10 mW cm) revealed a responsivity ( ) and external quantum efficiency (EQE) of 32.9 mA W and 120.2, respectively. Furthermore, a descended photocurrent behavior from 330 to 63.9 (μA) was observed at wavelengths of 340 and 625 nm with a visible light rejection ratio of 516%, indicating the visible blind characteristic of the proposed geometry. This was also observed at an extremely low bias potential (0.01 V). The incident power profile demonstrated an inversely proportional correlation to and EQE, with values 37.8 mA W and 137.7 at 6 mW cm, respectively. Of the fabricated devices, the photodetector performance attained at 700 pulses, nm, and 10 mW cm depicted a substantially rapid time-resolved characteristic with a rise and fall time of 0.29 and 0.31 s, respectively.

摘要

在本研究中,通过脉冲激光沉积(PLD)制备了一种纳米结构的氧化锡(IV)(SnO)/硅异质结紫外光电探测器,以响应激光脉冲。特别地,考虑到多轮廓依赖性,即激光脉冲、光谱响应和入射功率,对所提出器件的光电探测机制进行了深入研究。详细地说,由于脉冲数从300增加到700,出现了粒径为25和41 nm、带隙变化0.2 eV以及在335 nm左右的截止现象。最佳光电探测器(在700个脉冲、 nm和10 mW/cm²时)的响应度( )和外量子效率(EQE)分别为32.9 mA/W和120.2。此外,在波长为340和625 nm时观察到光电流行为从330下降到63.9(μA),可见光抑制比为516%,表明所提出结构具有可见光盲特性。在极低偏置电势(0.01 V)下也观察到了这一点。入射功率分布与 和EQE呈反比关系,在6 mW/cm²时的值分别为37.8 mA/W和137.7。在所制备的器件中,在700个脉冲、 nm和10 mW/cm²时获得的光电探测器性能表现出显著快速的时间分辨特性,上升时间和下降时间分别为0.29和0.31 s。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/ea80f020eaa1/d4ra05303f-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/bb50989f5ed6/d4ra05303f-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/fc99307b1ddc/d4ra05303f-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/9c41b27f4b81/d4ra05303f-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/f5002c2323c4/d4ra05303f-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/9567734eec04/d4ra05303f-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/ea80f020eaa1/d4ra05303f-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/bb50989f5ed6/d4ra05303f-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/fc99307b1ddc/d4ra05303f-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/9c41b27f4b81/d4ra05303f-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/f5002c2323c4/d4ra05303f-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/9567734eec04/d4ra05303f-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b50b/11367619/ea80f020eaa1/d4ra05303f-f6.jpg

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本文引用的文献

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用于高效稳定n-i-p钙钛矿太阳能电池的SnO研究进展。
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