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用于生物和水样中吡啶二甲酸传感的发光金属有机框架（MOF）的合成与应用：综述

Synthesis and applications of luminescent metal organic frameworks (MOFs) for sensing dipicolinic acid in biological and water samples: a review.

作者信息

Kayani Kawan F, Shatery Omer B A, Mohammed Sewara J, Ahmed Harez Rashid, Hamarawf Rebaz F, Mustafa Muhammad S

机构信息

Department of Chemistry, College of Science, Charmo University Peshawa Street, Chamchamal Sulaimani City 46023 Iraq.

Department of Chemistry, College of Science, University of Sulaimani Qliasan St 46002 Sulaimani City Kurdistan Region Iraq

出版信息

Nanoscale Adv. 2024 Nov 21;7(1):13-41. doi: 10.1039/d4na00652f. eCollection 2024 Dec 17.

DOI:10.1039/d4na00652f
PMID:39583129
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11579904/
Abstract

The detection of trace quantities of 2,6-dipicolinic acid (DPA) in real-world samples is crucial for early disease diagnosis and routine health monitoring. Metal-organic frameworks (MOFs), recognized for their diverse structural architectures, have emerged as advanced multifunctional hybrid materials. One of the most notable properties of MOFs is their luminescence (L), which can arise from structural ligands, guest molecules, and emissive metal ions. Luminescent MOFs have shown significant promise as platforms for sensor design. This review highlights the application of luminescent MOFs in the detection of DPA in biological and aqueous environments. It provides a comprehensive discussion of the various detection strategies employed in luminescent MOF-based DPA sensors. Additionally, it explores the origins of L in MOFs, their synthesis, and the mechanisms underlying their sensing capabilities. The article also addresses key challenges and limitations in this field, offering practical insights for the development of efficient luminescent MOFs for DPA detection.

摘要

在实际样品中检测痕量的2,6 - 二吡啶甲酸（DPA）对于早期疾病诊断和常规健康监测至关重要。金属有机框架（MOF）因其多样的结构架构而被认可，已成为先进的多功能杂化材料。MOF最显著的特性之一是其发光（L），这可能源于结构配体、客体分子和发光金属离子。发光MOF作为传感器设计平台已显示出巨大潜力。本综述重点介绍了发光MOF在生物和水环境中检测DPA的应用。它全面讨论了基于发光MOF的DPA传感器所采用的各种检测策略。此外，还探讨了MOF中发光的起源、它们的合成以及其传感能力的潜在机制。本文还讨论了该领域的关键挑战和局限性，为开发用于DPA检测的高效发光MOF提供了实用见解。

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