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二氧化碳捕集:可扩展材料与可持续解决方案的综合综述及文献计量分析

CO Capture: A Comprehensive Review and Bibliometric Analysis of Scalable Materials and Sustainable Solutions.

作者信息

Carrascal-Hernández Domingo Cesar, Grande-Tovar Carlos David, Mendez-Lopez Maximiliano, Insuasty Daniel, García-Freites Samira, Sanjuan Marco, Márquez Edgar

机构信息

Departamento de Química y Biología, Facultad de Ciencias Básicas, Universidad del Norte, Barranquilla 080020, Colombia.

Grupo de Investigación de Fotoquímica y Fotobiología, Programa de Química, Universidad del Atlántico, Carrera 30 No 8-49, Puerto Colombia 081007, Colombia.

出版信息

Molecules. 2025 Jan 26;30(3):563. doi: 10.3390/molecules30030563.

Abstract

The greenhouse effect and global warming, driven by the accumulation of pollutants, such as sulfur oxides (SOx), nitrogen oxides (NOx), and CO, are primarily caused by the combustion of fossil fuels and volcanic eruptions. These phenomena represent an international crisis that negatively impacts human health and the environment. Several studies have reported novel carbon capture, utilization, and storage (CCUS) technologies, promising solutions. Notable methods include chemical absorption using solvents, and the development of functionalized porous materials, such as MCM-41, impregnated with amines like polyethyleneimine. These technologies have demonstrated high capture capacity and thermal stability; however, they face challenges related to recyclability and high operating costs. In parallel, biodegradable polymers and hydrogels present sustainable alternatives with a lower environmental impact, although their industrial scalability remains limited. This review comprehensively analyzes CO capture methods, focusing on silica-based porous supports, polymers, hydrogels, and emerging techniques, like CCUS and MOFs, while including traditional methods and a bibliometric analysis to update the field's scientific dynamics. With increasing investigations focused on developing new CCUS technologies, this study highlights a growing interest in eco-friendly alternatives. A bibliometric analysis of 903 articles published between 2010 and 2024 provides an overview of current research on environmentally friendly carbon capture technologies. Countries such as the United States, the United Kingdom, and India are leading research efforts in this field, emphasizing the importance of scientific collaboration. Despite these advancements, implementing these technologies in industrial sectors with high greenhouse gas emissions remains scarce. This underscores the need for public policies and financing to promote their development and application in these sectors. Future research should prioritize materials with high capture capacity, efficient transformation, and valorization of CO while promoting circular economy approaches and decarbonizing challenging sectors, such as energy and transportation. Integrating environmentally friendly materials, energy optimization, and sustainable strategies is essential to position these technologies as key tools in the fight against climate change.

摘要

由硫氧化物(SOx)、氮氧化物(NOx)和一氧化碳等污染物的积累所驱动的温室效应和全球变暖,主要是由化石燃料燃烧和火山喷发引起的。这些现象构成了一场对人类健康和环境产生负面影响的国际危机。多项研究报告了新型碳捕获、利用和储存(CCUS)技术,这些技术是很有前景的解决方案。值得注意的方法包括使用溶剂进行化学吸收,以及开发功能化多孔材料,如浸渍有聚乙烯亚胺等胺类的MCM - 41。这些技术已展现出高捕获能力和热稳定性;然而,它们面临着与可回收性和高运营成本相关的挑战。与此同时,可生物降解聚合物和水凝胶提供了具有较低环境影响的可持续替代方案,尽管它们的工业可扩展性仍然有限。本综述全面分析了二氧化碳捕获方法,重点关注基于二氧化硅的多孔载体、聚合物、水凝胶以及新兴技术,如CCUS和金属有机框架(MOF),同时涵盖传统方法并进行文献计量分析以更新该领域的科学动态。随着越来越多的研究聚焦于开发新的CCUS技术,本研究凸显了对环保替代方案的兴趣日益浓厚。对2010年至2024年间发表的903篇文章进行的文献计量分析概述了当前对环境友好型碳捕获技术的研究。美国、英国和印度等国家在该领域引领研究工作,强调了科学合作的重要性。尽管取得了这些进展,但在温室气体排放量大的工业部门中实施这些技术的情况仍然很少。这凸显了需要公共政策和资金来促进它们在这些部门的开发和应用。未来的研究应优先考虑具有高捕获能力、高效转化以及二氧化碳增值的材料,同时推广循环经济方法并使能源和交通等具有挑战性的部门脱碳。整合环境友好型材料、能源优化和可持续战略对于将这些技术定位为应对气候变化的关键工具至关重要。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6510/11820267/f2e4ad038e43/molecules-30-00563-g007.jpg

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