Metal-Organic Framework-Based Micro-/Nanomotors for Wastewater Remediation.

Micro-/nanomotors (MNMs) in water remediation have garnered significant attention over the past two decades. More recently, metal-organic framework-based micro-/nanomotors (MOF-MNMs) have been applied for environmental remediation; however, a comprehensive summary of research in this research area is yet to be reported. Herein, a review is presented to cover the recent advances in MOF-MNMs and their various applications in wastewater remediation. The review presents a comprehensive introduction to MNMs, including different propulsion approaches, fabrication, and functionalization strategies, in addition to the unique features of MOF-MNMs. The conception and various synthetic routes of MOF-MNMs are extensively covered and the implementation of MOF-MNMs in water-related applications, including adsorption, degradation, sensing, and disinfection of different pollutants, is in depth discussed. Meanwhile, the propulsion and mechanism of action behind each MOF-MNM are systematically studied. Finally, the review provides insights into the challenges and perspectives to build more effective MOF-MNMs to cover versatile applications for wastewater treatment.