Hossain Md Anik, Illescas-Lopez Sara, Firouzeh Seyedamin, Cuerva Juan Manuel, de Cienfuegos Luis Álvarez, Pramanik Sandipan
Department of Electrical and Computer Engineering, University of Alberta, Edmonton, Alberta T6G 1H9, Canada.
Universidad de Granada, Departamento de Química Orgánica, Unidad de Excelencia Química Aplicada a Biomedicina y Medioambiente, C. U. Fuentenueva, Avda. Severo Ochoa s/n, E-18071 Granada, Spain.
Nano Lett. 2025 Jun 18;25(24):9623-9630. doi: 10.1021/acs.nanolett.5c01297. Epub 2025 Jun 9.
Chiral materials contacted between a ferromagnet (FM) and a nonmagnet (NM) exhibit a chirality-dependent asymmetric magnetoresistance (MR) as the FM magnetization is flipped. This is considered to be a manifestation of the chirality induced spin selectivity (CISS) effect, in which chirality dependent spins generated in the medium are subsequently detected by the ferromagnetic spin detector. Here we show that this two-terminal asymmetric MR response is quite general and can arise even when an medium is contacted by electrodes, with no known spin detecting property. By controllably introducing chirality in the channel, we demonstrate how the CISS MR manifests . The response, distinct from electromagnetochiral anisotropy (EMChA), remains unchanged in the standard configuration with FM/NM electrodes. Thus, observation of chirality-dependent MR in transport experiments does not necessarily relate chirality to spin, as commonly assumed in CISS literature.
当铁磁体(FM)和非磁体(NM)接触时,手性材料会在FM磁化翻转时表现出与手性相关的不对称磁电阻(MR)。这被认为是手性诱导自旋选择性(CISS)效应的一种表现,在该效应中,介质中产生的与手性相关的自旋随后被铁磁自旋探测器检测到。在这里,我们表明这种两端不对称MR响应非常普遍,即使在没有已知自旋检测特性的电极接触介质时也可能出现。通过可控地在通道中引入手性,我们展示了CISS MR是如何表现的。这种响应与电磁手性各向异性(EMChA)不同,在FM/NM电极的标准配置中保持不变。因此,在输运实验中观察到的与手性相关的MR不一定像CISS文献中通常假设的那样将手性与自旋联系起来。