Meador Danielle S, Houck Stephanie S, Spivak David A
Department of Chemistry, Louisiana State University, Baton Rouge, LA 70803, USA.
Parkersburg High School, 2101 Dudley Ave, Parkersburg, WV 26101, USA.
Polymers (Basel). 2025 Aug 30;17(17):2359. doi: 10.3390/polym17172359.
Molecularly imprinted polymers (MIPs) are polymeric receptors for a targeted template molecule that are traditionally formed using a combination of functional monomers and crosslinkers. While investigating novel crosslinkers for MIPs, one of these (2-(methacryloylamino)ethyl-2-methylacrylate (referred to as N,O-bismethacryloyl ethanolamine or "NOBE")) performed better when used alone versus in combination with other monomers. This introduced the concept of one monomer molecularly imprinted polymers, given the acronym OMNiMIPs, and prompted studies provided in this report that clarify OMNiMIPs have fundamental differences compared to traditionally formulated MIPs. Enantioselectivity studies using BOC-L-tyrosine as a standard template showed that NOBE OMNiMIPs afforded higher-performing MIPs compared with traditional MIPs, have significantly higher binding capacities, and have an internal hydrogen-bonded crosslinking structure that contributes to the morphological stability of the binding site structure. Based on the adventitious discovery of NOBE OMNiMIPs, new analogs based on the NOBE structure were developed and evaluated for further enhancement of molecular recognition performance and novel capabilities of OMNiMIPs. While the majority of the new OMNiMIPs exhibited enantiomeric selectivity toward BOC-L-tyr, improvements were not observed compared with NOBE.
分子印迹聚合物(MIPs)是针对目标模板分子的聚合物受体,传统上是使用功能单体和交联剂的组合形成的。在研究MIPs的新型交联剂时,其中一种(2-(甲基丙烯酰氨基)乙基-2-甲基丙烯酸酯(称为N,O-双甲基丙烯酰乙醇胺或“NOBE”))单独使用时比与其他单体组合使用时表现更好。这引入了一种单体分子印迹聚合物的概念,简称为OMNiMIPs,并促使本报告中的研究得以开展,这些研究阐明了OMNiMIPs与传统配方的MIPs相比存在根本差异。以BOC-L-酪氨酸作为标准模板的对映选择性研究表明,与传统MIPs相比,NOBE OMNiMIPs提供了性能更高的MIPs,具有显著更高的结合能力,并且具有内部氢键交联结构,这有助于结合位点结构的形态稳定性。基于NOBE OMNiMIPs的偶然发现,开发并评估了基于NOBE结构的新类似物,以进一步提高分子识别性能和OMNiMIPs的新功能。虽然大多数新的OMNiMIPs对BOC-L- tyr表现出对映体选择性,但与NOBE相比未观察到改善。