Zhan Shuming, Wang Chengyu, Duan Longhui, Gu Zhenhua
Department of Chemistry, University of Science and Technology of China 96 Jinzhai Road Hefei Anhui 230026 P. R. China.
State Key Laboratory of Coordination Chemistry, Nanjing University Nanjing 210093 P. R. China
Chem Sci. 2025 Sep 17. doi: 10.1039/d5sc03779d.
The [2.2.1]-bridged bicyclic framework represents a privileged structural motif prevalent in numerous bioactive molecules and functional materials. The development of efficient synthetic methods for constructing these valuable architectures remains highly desirable. In this study, we report a dirhodium(ii)/bisphosphine-catalyzed desymmetrization reaction of benzobicyclo[2.2.1]heptane-2,3-diones with arylboronic acids. This transformation delivers enantioenriched benzo[2.2.1] α-hydroxy ketones with excellent enantioselectivity (up to 94% ee) across a diverse substrate scope. The synthetic utility of these chiral products is demonstrated through several transformations, including the preparation of a chiral phosphine.
[2.2.1]桥连双环骨架是众多生物活性分子和功能材料中普遍存在的一种优势结构基序。开发用于构建这些有价值结构的高效合成方法仍然非常必要。在本研究中,我们报道了一种二铑(II)/双膦催化的苯并双环[2.2.1]庚烷-2,3-二酮与芳基硼酸的去对称化反应。该转化反应在广泛的底物范围内以优异的对映选择性(高达94%ee)提供对映体富集的苯并[2.2.1]α-羟基酮。通过包括制备手性膦在内的几种转化反应,证明了这些手性产物的合成实用性。