Sugishima Masakazu, Migita Catharina T, Zhang Xuhong, Yoshida Tadashi, Fukuyama Keiichi
Department of Biology, Graduate School of Science, Osaka University, Toyonaka, Osaka, Japan.
Eur J Biochem. 2004 Nov;271(22):4517-25. doi: 10.1111/j.1432-1033.2004.04411.x.
Heme oxygenase (HO) catalyzes the oxidative degradation of heme utilizing molecular oxygen and reducing equivalents. In photosynthetic organisms, HO functions in the biosynthesis of such open-chain tetrapyrroles as phyto-chromobilin and phycobilins, which are involved in the signal transduction for light responses and light harvesting for photosynthesis, respectively. We have determined the first crystal structure of a HO-1 from a photosynthetic organism, Synechocystis sp. PCC 6803 (Syn HO-1), in complex with heme at 2.5 A resolution. Heme-Syn HO-1 shares a common folding with other heme-HOs. Although the heme pocket of heme-Syn HO-1 is, for the most part, similar to that of mammalian HO-1, they differ in such features as the flexibility of the distal helix and hydrophobicity. In addition, 2-propanol derived from the crystallization solution occupied the hydrophobic cavity, which is proposed to be a CO trapping site in rat HO-1 that suppresses product inhibition. Although Syn HO-1 and mammalian HO-1 are similar in overall structure and amino acid sequence (57% similarity vs. human HO-1), their molecular surfaces differ in charge distribution. The surfaces of the heme binding sides are both positively charged, but this patch of Syn HO-1 is narrow compared to that of mammalian HO-1. This feature is suited to the selective binding of ferredoxin, the physiological redox partner of Syn HO-1; the molecular size of ferredoxin is approximately 10 kDa whereas the size of NADPH-cytochrome P450 reductase, a reducing partner of mammalian HO-1, is approximately 77 kDa. A docking model of heme-Syn HO-1 and ferredoxin suggests indirect electron transfer from an iron-sulfur cluster in ferredoxin to the heme iron of heme-Syn HO-1.
血红素加氧酶(HO)利用分子氧和还原当量催化血红素的氧化降解。在光合生物中,HO在诸如植物色素胆素和藻胆素等开链四吡咯的生物合成中发挥作用,它们分别参与光反应的信号转导和光合作用的光捕获。我们已经确定了来自光合生物集胞藻PCC 6803(Syn HO-1)的HO-1与血红素复合物的首个晶体结构,分辨率为2.5埃。血红素-Syn HO-1与其他血红素-HO具有共同的折叠方式。尽管血红素-Syn HO-1的血红素口袋在很大程度上与哺乳动物HO-1的相似,但它们在诸如远端螺旋的柔韧性和疏水性等特征上有所不同。此外,来自结晶溶液的2-丙醇占据了疏水腔,该疏水腔被认为是大鼠HO-1中抑制产物抑制的CO捕获位点。尽管Syn HO-1和哺乳动物HO-1在整体结构和氨基酸序列上相似(与人类HO-1的相似度为57%),但它们的分子表面电荷分布不同。血红素结合侧的表面均带正电荷,但与哺乳动物HO-1相比,Syn HO-1的这片区域较窄。这一特征适合于铁氧还蛋白(Syn HO-1的生理氧化还原伙伴)的选择性结合;铁氧还蛋白的分子大小约为10 kDa,而哺乳动物HO-1的还原伙伴NADPH-细胞色素P450还原酶的大小约为77 kDa。血红素-Syn HO-1与铁氧还蛋白的对接模型表明,电子从铁氧还蛋白中的铁硫簇间接转移至血红素-Syn HO-1的血红素铁。