Richter Andreas, Burrows John P, Nüss Hendrik, Granier Claire, Niemeier Ulrike
Institute of Environmental Physics, University of Bremen, Otto-Hahn-Allee 1, D-28359 Bremen, Germany.
Nature. 2005 Sep 1;437(7055):129-32. doi: 10.1038/nature04092.
Emissions from fossil fuel combustion and biomass burning reduce local air quality and affect global tropospheric chemistry. Nitrogen oxides are emitted by all combustion processes and play a key part in the photochemically induced catalytic production of ozone, which results in summer smog and has increased levels of tropospheric ozone globally. Release of nitrogen oxide also results in nitric acid deposition, and--at least locally--increases radiative forcing effects due to the absorption of downward propagating visible light. Nitrogen oxide concentrations in many industrialized countries are expected to decrease, but rapid economic development has the potential to increase significantly the emissions of nitrogen oxides in parts of Asia. Here we present the tropospheric column amounts of nitrogen dioxide retrieved from two satellite instruments GOME and SCIAMACHY over the years 1996-2004. We find substantial reductions in nitrogen dioxide concentrations over some areas of Europe and the USA, but a highly significant increase of about 50 per cent-with an accelerating trend in annual growth rate-over the industrial areas of China, more than recent bottom-up inventories suggest.
化石燃料燃烧和生物质燃烧排放会降低当地空气质量,并影响全球对流层化学。所有燃烧过程都会排放氮氧化物,其在光化学诱导的臭氧催化生成过程中起关键作用,这会导致夏季烟雾,并使全球对流层臭氧水平升高。氮氧化物的释放还会导致硝酸沉降,并且至少在局部地区,由于向下传播的可见光的吸收,会增加辐射强迫效应。预计许多工业化国家的氮氧化物浓度将会下降,但经济的快速发展有可能使亚洲部分地区的氮氧化物排放量大幅增加。在此,我们展示了利用两台卫星仪器GOME和SCIAMACHY在1996年至2004年期间获取的对流层二氧化氮柱总量。我们发现欧洲和美国部分地区的二氧化氮浓度大幅下降,但中国工业区的二氧化氮浓度显著增加了约50%,且年增长率呈加速趋势,这比近期的自下而上排放清单所显示的情况更为严重。