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天然聚醚类抗生素的结构与性质。

Structures and properties of naturally occurring polyether antibiotics.

机构信息

Department of Biochemistry, Faculty of Chemistry, Adam Mickiewicz University, Grunwaldzka 6, 60-780 Poznań, Poland.

出版信息

Biomed Res Int. 2013;2013:162513. doi: 10.1155/2013/162513. Epub 2013 Mar 17.

DOI:10.1155/2013/162513
PMID:23586016
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC3613094/
Abstract

Polyether ionophores represent a large group of natural, biologically active substances produced by Streptomyces spp. They are lipid soluble and able to transport metal cations across cell membranes. Several of polyether ionophores are widely used as growth promoters in veterinary. Polyether antibiotics show a broad spectrum of bioactivity ranging from antibacterial, antifungal, antiparasitic, antiviral, and tumour cell cytotoxicity. Recently, it has been shown that some of these compounds are able to selectively kill cancer stem cells and multidrug-resistant cancer cells. Thus, they are recognized as new potential anticancer drugs. The biological activity of polyether ionophores is strictly connected with their molecular structure; therefore, the purpose of this paper is to present an overview of their formula, molecular structure, and properties.

摘要

聚醚离子载体是一大类由链霉菌属（Streptomyces spp.）产生的天然、具有生物活性的物质。它们具有亲脂性，能够将金属阳离子穿过细胞膜进行运输。有几种聚醚离子载体被广泛用作兽医中的生长促进剂。聚醚抗生素表现出广泛的生物活性，包括抗菌、抗真菌、抗寄生虫、抗病毒和肿瘤细胞细胞毒性。最近，已经表明这些化合物中的一些能够选择性地杀死癌症干细胞和多药耐药性癌细胞。因此，它们被认为是新的潜在抗癌药物。聚醚离子载体的生物活性与它们的分子结构密切相关；因此，本文的目的是介绍它们的配方、分子结构和性质的概述。

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5
First solid state alkaline-earth complexes of monensic acid A (MonH): crystal structure of [M(Mon)2(H (2)O)2] (M = Mg, Ca), spectral properties and cytotoxicity against aerobic Gram-positive bacteria.首例固态碱土金属 monensic 酸 A（MonH）配合物：[M(Mon)2(H (2)O)2]（M = Mg, Ca）的晶体结构、光谱性质和对需氧革兰氏阳性菌的细胞毒性。
Biometals. 2010 Feb;23(1):59-70. doi: 10.1007/s10534-009-9269-5. Epub 2009 Sep 21.
6
Crystal structure and properties of the copper(II) complex of sodium monensin A.莫能菌素A钠铜（II）配合物的晶体结构与性质
J Inorg Biochem. 2009 Oct;103(10):1419-24. doi: 10.1016/j.jinorgbio.2009.08.007. Epub 2009 Aug 25.
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A synthesis of an ionomycin calcium complex.离子霉素钙复合物的合成。
Angew Chem Int Ed Engl. 2009;48(27):5022-5. doi: 10.1002/anie.200901608.
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First divalent metal complexes of the polyether ionophore Monensin A: X-Ray structures of [Co(Mon)2(H2O)2] and [Mn(Mon)2(H2O)2] and their bactericidal properties.聚醚离子载体莫能菌素A的首例二价金属配合物：[Co(Mon)2(H2O)2]和[Mn(Mon)2(H2O)2]的X射线结构及其杀菌性能
Curr Drug Discov Technol. 2008 Jun;5(2):154-61. doi: 10.2174/157016308784746247.
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Synthesis and antimicrobial properties of monensin A esters.莫能菌素A酯的合成及其抗菌性能
Bioorg Med Chem Lett. 2008 Apr 15;18(8):2585-9. doi: 10.1016/j.bmcl.2008.03.038. Epub 2008 Mar 16.
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Synthesis, structure and antimicrobial activity of manganese(II) and cobalt(II) complexes of the polyether ionophore antibiotic Sodium Monensin A.聚醚离子载体抗生素莫能菌素A钠的锰（II）和钴（II）配合物的合成、结构及抗菌活性
J Inorg Biochem. 2008 Jan;102(1):26-32. doi: 10.1016/j.jinorgbio.2007.06.033. Epub 2007 Jul 1.