Department of Physics and Texas Center for Superconductivity, University of Houston, Houston, TX 77204, USA.
Proc Natl Acad Sci U S A. 2013 Aug 13;110(33):13261-6. doi: 10.1073/pnas.1305735110. Epub 2013 Jul 30.
From an environmental perspective, lead-free SnTe would be preferable for solid-state waste heat recovery if its thermoelectric figure-of-merit could be brought close to that of the lead-containing chalcogenides. In this work, we studied the thermoelectric properties of nanostructured SnTe with different dopants, and found indium-doped SnTe showed extraordinarily large Seebeck coefficients that cannot be explained properly by the conventional two-valence band model. We attributed this enhancement of Seebeck coefficients to resonant levels created by the indium impurities inside the valence band, supported by the first-principles simulations. This, together with the lower thermal conductivity resulting from the decreased grain size by ball milling and hot pressing, improved both the peak and average nondimensional figure-of-merit (ZT) significantly. A peak ZT of ∼1.1 was obtained in 0.25 atom % In-doped SnTe at about 873 K.
从环境角度来看,如果无铅 SnTe 的热电优值能接近含铅的硫族化物,那么它将更适合用于固态废热回收。在这项工作中,我们研究了具有不同掺杂剂的纳米结构 SnTe 的热电性能,发现掺铟 SnTe 表现出异常大的 Seebeck 系数,这不能用传统的两能带模型来很好地解释。我们将这种 Seebeck 系数的增强归因于价带内铟杂质所产生的共振能级,这一观点得到了第一性原理模拟的支持。这一点,再加上通过球磨和热压减小晶粒尺寸导致的热导率降低,显著提高了峰和平均无量纲优值(ZT)。在约 873 K 时,在 0.25 原子%的 In 掺杂 SnTe 中获得了约 1.1 的峰值 ZT。