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高质量单层和双层 MoS2 的本征电子输运性质。

Intrinsic electronic transport properties of high-quality monolayer and bilayer MoS2.

机构信息

Department of Physics, Massachusetts Institute of Technology , 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, United States.

出版信息

Nano Lett. 2013 Sep 11;13(9):4212-6. doi: 10.1021/nl401916s. Epub 2013 Aug 20.

Abstract

We report electronic transport measurements of devices based on monolayers and bilayers of the transition-metal dichalcogenide MoS2. Through a combination of in situ vacuum annealing and electrostatic gating we obtained ohmic contact to the MoS2 down to 4 K at high carrier densities. At lower carrier densities, low-temperature four probe transport measurements show a metal-insulator transition in both monolayer and bilayer samples. In the metallic regime, the high-temperature behavior of the mobility showed strong temperature dependence consistent with phonon-dominated transport. At low temperature, intrinsic field-effect mobilities approaching 1000 cm(2)/(V·s) were observed for both monolayer and bilayer devices. Mobilities extracted from Hall effect measurements were several times lower and showed a strong dependence on density, likely caused by screening of charged impurity scattering at higher densities.

摘要

我们报告了基于过渡金属二硫化物 MoS2 的单层和双层器件的电子输运测量结果。通过原位真空退火和静电门控的组合,我们在高载流子密度下获得了低至 4 K 的 MoS2 的欧姆接触。在较低的载流子密度下,低温四探针输运测量显示单层和双层样品均发生金属-绝缘体转变。在金属态,迁移率的高温行为表现出与声子主导输运一致的强烈温度依赖性。在低温下,单层和双层器件均观察到接近 1000 cm(2)/(V·s)的本征场效应迁移率。霍尔效应测量得出的迁移率要低几个数量级,并且强烈依赖于密度,这可能是由于在较高密度下屏蔽了带电杂质散射。

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