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美国生产高粱生物乙醇的生命周期能源利用和温室气体排放。

Life-cycle energy use and greenhouse gas emissions of production of bioethanol from sorghum in the United States.

机构信息

Systems Assessment Group, Energy Systems Division, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439, USA.

出版信息

Biotechnol Biofuels. 2013 Oct 2;6(1):141. doi: 10.1186/1754-6834-6-141.

Abstract

BACKGROUND

The availability of feedstock options is a key to meeting the volumetric requirement of 136.3 billion liters of renewable fuels per year beginning in 2022, as required in the US 2007 Energy Independence and Security Act. Life-cycle greenhouse gas (GHG) emissions of sorghum-based ethanol need to be assessed for sorghum to play a role in meeting that requirement.

RESULTS

Multiple sorghum-based ethanol production pathways show diverse well-to-wheels (WTW) energy use and GHG emissions due to differences in energy use and fertilizer use intensity associated with sorghum growth and differences in the ethanol conversion processes. All sorghum-based ethanol pathways can achieve significant fossil energy savings. Relative to GHG emissions from conventional gasoline, grain sorghum-based ethanol can reduce WTW GHG emissions by 35% or 23%, respectively, when wet or dried distillers grains with solubles (DGS) is the co-product and fossil natural gas (FNG) is consumed as the process fuel. The reduction increased to 56% or 55%, respectively, for wet or dried DGS co-production when renewable natural gas (RNG) from anaerobic digestion of animal waste is used as the process fuel. These results do not include land-use change (LUC) GHG emissions, which we take as negligible. If LUC GHG emissions for grain sorghum ethanol as estimated by the US Environmental Protection Agency (EPA) are included (26 g CO2e/MJ), these reductions when wet DGS is co-produced decrease to 7% or 29% when FNG or RNG is used as the process fuel. Sweet sorghum-based ethanol can reduce GHG emissions by 71% or 72% without or with use of co-produced vinasse as farm fertilizer, respectively, in ethanol plants using only sugar juice to produce ethanol. If both sugar and cellulosic bagasse were used in the future for ethanol production, an ethanol plant with a combined heat and power (CHP) system that supplies all process energy can achieve a GHG emission reduction of 70% or 72%, respectively, without or with vinasse fertigation. Forage sorghum-based ethanol can achieve a 49% WTW GHG emission reduction when ethanol plants meet process energy demands with CHP. In the case of forage sorghum and an integrated sweet sorghum pathway, the use of a portion of feedstock to fuel CHP systems significantly reduces fossil fuel consumption and GHG emissions.

CONCLUSIONS

This study provides new insight into life-cycle energy use and GHG emissions of multiple sorghum-based ethanol production pathways in the US. Our results show that adding sorghum feedstocks to the existing options for ethanol production could help in meeting the requirements for volumes of renewable, advanced and cellulosic bioethanol production in the US required by the EPA's Renewable Fuel Standard program.

摘要

背景

为了满足美国 2007 年《能源独立与安全法案》规定的从 2022 年开始每年需生产 1363 亿升可再生燃料的体积要求,原料选择至关重要。为了使高粱在满足这一要求方面发挥作用,需要评估基于高粱的乙醇的生命周期温室气体(GHG)排放。

结果

由于高粱生长过程中能源使用和肥料使用强度的差异以及乙醇转化过程的差异,多种基于高粱的乙醇生产途径的全生命周期(WTW)能源使用和 GHG 排放存在差异。所有基于高粱的乙醇途径都可以实现显著的化石能源节约。与传统汽油相比,当湿或干酒糟及其可溶物(DGS)是共产物且化石天然气(FNG)用作工艺燃料时,基于粮食高粱的乙醇分别可以减少 35%或 23%的 WTW GHG 排放。当使用动物废物厌氧消化产生的可再生天然气(RNG)作为工艺燃料时,湿或干 DGS 共生产的减少量分别增加到 56%或 55%。这些结果不包括土地利用变化(LUC)GHG 排放,我们认为这些排放可以忽略不计。如果包括美国环境保护署(EPA)估计的粮食高粱乙醇的 LUC GHG 排放(26 g CO2e/MJ),当使用 FNG 或 RNG 作为工艺燃料时,当湿 DGS 共生产时,这些减少量分别降低到 7%或 29%。仅使用糖汁生产乙醇的乙醇工厂,如果使用共生产的酒糟作为农场肥料,甜高粱基乙醇可以分别减少 71%或 72%的 GHG 排放。如果未来同时使用糖和纤维素甘蔗渣用于乙醇生产,配备热电联产(CHP)系统的乙醇工厂可以在不使用酒糟施肥的情况下分别实现 70%或 72%的 GHG 减排,或者在使用酒糟施肥的情况下实现 70%或 72%的 GHG 减排。对于饲料高粱基乙醇,当乙醇工厂使用 CHP 满足工艺能源需求时,其全生命周期 GHG 排放可减少 49%。在饲料高粱和综合甜高粱途径的情况下,使用一部分原料为 CHP 系统提供燃料可以显著减少化石燃料消耗和 GHG 排放。

结论

本研究为美国多种基于高粱的乙醇生产途径的生命周期能源利用和 GHG 排放提供了新的见解。我们的研究结果表明,在美国 EPA 的可再生燃料标准计划规定的先进和纤维素生物乙醇生产所需的可再生、先进和纤维素生物乙醇的数量要求下,增加高粱原料的选择可能有助于满足要求。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/efd7/3850671/19ab23a85b1b/1754-6834-6-141-1.jpg

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