IBM Thomas J. Watson Research Center, Yorktown Heights, New York 10598, United States.
Nano Lett. 2014 Aug 13;14(8):4581-6. doi: 10.1021/nl501628x. Epub 2014 Jul 16.
In the phenomenon of plasmon-induced transparency, which is a classical analogue of electromagnetically induced transparency (EIT) in atomic gases, the coherent interference between two plasmon modes results in an optical transparency window in a broad absorption spectrum. With the requirement of contrasting lifetimes, typically one of the plasmon modes involved is a dark mode that has limited coupling to the electromagnetic radiation and possesses relatively longer lifetime. Plasmon-induced transparency not only leads to light transmission at otherwise opaque frequency regions but also results in the slowing of light group velocity and enhanced optical nonlinearity. In this article, we report an analogous behavior, denoted as phonon-induced transparency (PIT), in AB-stacked bilayer graphene nanoribbons. Here, light absorption due to the plasmon excitation is suppressed in a narrow window due to the coupling with the infrared active Γ-point optical phonon, whose function here is similar to that of the dark plasmon mode in the plasmon-induced transparency. We further show that PIT in bilayer graphene is actively tunable by electrostatic gating and estimate a maximum slow light factor of around 500 at the phonon frequency of 1580 cm(-1), based on the measured spectra. Our demonstration opens an avenue for the exploration of few-photon nonlinear optics and slow light in this novel two-dimensional material.
在等离子体诱导透明现象中,这是原子气体中电磁感应透明(EIT)的经典模拟,两个等离子体模式之间的相干干涉导致在宽吸收光谱中出现光学透明窗口。由于寿命对比的要求,所涉及的等离子体模式之一通常是暗模式,其与电磁辐射的耦合有限,并且具有相对较长的寿命。等离子体诱导透明不仅导致在原本不透明的频率区域中的光传输,而且导致光群速度的减慢和光学非线性的增强。在本文中,我们在 AB 堆叠双层石墨烯纳米带中报告了类似的行为,称为声子诱导透明(PIT)。在这里,由于与红外活动的Γ点光学声子的耦合,等离子体激发引起的光吸收在窄窗口中被抑制,其功能类似于等离子体诱导透明中的暗等离子体模式。我们进一步表明,双层石墨烯中的 PIT 可以通过静电门控进行主动调谐,并根据测量的光谱估计在声子频率为 1580cm(-1) 时最大慢光因子约为 500。我们的演示为在这种新型二维材料中探索少光子非线性光学和慢光开辟了一条途径。