van der Sar Toeno, Casola Francesco, Walsworth Ronald, Yacoby Amir
Department of Physics, Harvard University, 17 Oxford St., Cambridge, Massachusetts 02138, USA.
1] Department of Physics, Harvard University, 17 Oxford St., Cambridge, Massachusetts 02138, USA [2] Harvard-Smithsonian Centre for Astrophysics, 60 Garden St., Cambridge, Massachusetts 02138, USA.
Nat Commun. 2015 Aug 7;6:7886. doi: 10.1038/ncomms8886.
Pushing the frontiers of condensed-matter magnetism requires the development of tools that provide real-space, few-nanometre-scale probing of correlated-electron magnetic excitations under ambient conditions. Here we present a practical approach to meet this challenge, using magnetometry based on single nitrogen-vacancy centres in diamond. We focus on spin-wave excitations in a ferromagnetic microdisc, and demonstrate local, quantitative and phase-sensitive detection of the spin-wave magnetic field at ∼50 nm from the disc. We map the magnetic-field dependence of spin-wave excitations by detecting the associated local reduction in the disc's longitudinal magnetization. In addition, we characterize the spin-noise spectrum by nitrogen-vacancy spin relaxometry, finding excellent agreement with a general analytical description of the stray fields produced by spin-spin correlations in a 2D magnetic system. These complementary measurement modalities pave the way towards imaging the local excitations of systems such as ferromagnets and antiferromagnets, skyrmions, atomically assembled quantum magnets, and spin ice.
拓展凝聚态磁学的前沿领域需要开发能在环境条件下对关联电子磁激发进行实空间、几纳米尺度探测的工具。在此,我们提出一种实用方法来应对这一挑战,即利用基于金刚石中单个氮空位中心的磁力测量法。我们聚焦于铁磁微盘中的自旋波激发,并展示了在距圆盘约50纳米处对自旋波磁场进行局部、定量和相位敏感检测。我们通过检测圆盘中纵向磁化强度的相关局部降低来绘制自旋波激发的磁场依赖性。此外,我们通过氮空位自旋弛豫测量法对自旋噪声谱进行了表征,发现与二维磁系统中自旋 - 自旋相关性产生的杂散场的一般解析描述非常吻合。这些互补的测量方式为成像诸如铁磁体和反铁磁体、斯格明子、原子组装量子磁体以及自旋冰等系统的局部激发铺平了道路。