Al-Ta'ii Hassan Maktuff Jaber, Periasamy Vengadesh, Amin Yusoff Mohd
Low Dimensional Materials Research Centre (LDMRC), Department of Physics, Faculty of Science, University of Malaya, 50603 Kuala Lumpur, Malaysia.
Department of Physics, Faculty of Science, University of Al-Muthana, Al-Muthana 66001, Iraq.
PLoS One. 2016 Jan 22;11(1):e0145423. doi: 10.1371/journal.pone.0145423. eCollection 2016.
Deoxyribonucleic acid or DNA molecules expressed as double-stranded (DSS) negatively charged polymer plays a significant role in electronic states of metal/silicon semiconductor structures. Electrical parameters of an Au/DNA/ITO device prepared using self-assembly method was studied by using current-voltage (I-V) characteristic measurements under alpha bombardment at room temperature. The results were analyzed using conventional thermionic emission model, Cheung and Cheung's method and Norde's technique to estimate the barrier height, ideality factor, series resistance and Richardson constant of the Au/DNA/ITO structure. Besides demonstrating a strongly rectifying (diode) characteristic, it was also observed that orderly fluctuations occur in various electrical parameters of the Schottky structure. Increasing alpha radiation effectively influences the series resistance, while the barrier height, ideality factor and interface state density parameters respond linearly. Barrier height determined from I-V measurements were calculated at 0.7284 eV for non-radiated, increasing to about 0.7883 eV in 0.036 Gy showing an increase for all doses. We also demonstrate the hypersensitivity phenomena effect by studying the relationship between the series resistance for the three methods, the ideality factor and low-dose radiation. Based on the results, sensitive alpha particle detectors can be realized using Au/DNA/ITO Schottky junction sensor.
脱氧核糖核酸或DNA分子以双链(DSS)带负电荷的聚合物形式存在,在金属/硅半导体结构的电子态中起着重要作用。通过在室温下α轰击下的电流-电压(I-V)特性测量,研究了采用自组装方法制备的Au/DNA/ITO器件的电学参数。使用传统的热电子发射模型、Cheung和Cheung方法以及Norde技术对结果进行分析,以估计Au/DNA/ITO结构的势垒高度、理想因子、串联电阻和理查森常数。除了表现出强烈的整流(二极管)特性外,还观察到肖特基结构的各种电学参数出现有序波动。增加α辐射有效地影响串联电阻,而势垒高度、理想因子和界面态密度参数呈线性响应。根据I-V测量确定的势垒高度,对于未辐射的情况计算为0.7284 eV,在0.036 Gy时增加到约0.7883 eV,表明所有剂量下均增加。我们还通过研究三种方法的串联电阻、理想因子与低剂量辐射之间的关系,证明了超敏现象效应。基于这些结果,可以使用Au/DNA/ITO肖特基结传感器实现灵敏的α粒子探测器。