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垂直堆叠石墨烯/单层 n-MoS/SiO/p-GaN 异质结构的多样化功能。

Diverse Functionalities of Vertically Stacked Graphene/Single layer n-MoS/SiO/p-GaN Heterostructures.

机构信息

Department of Physics, National Taiwan University, Taipei, 106, Taiwan.

Nano Science and Technology Program, Taiwan International Graduate Program, Academia Sinica and National Taiwan University, Taipei, 106, Taiwan.

出版信息

Sci Rep. 2017 Aug 30;7(1):10002. doi: 10.1038/s41598-017-09998-1.

Abstract

Integrating different dimentional materials on vertically stacked p-n hetero-junctions have facinated a considerable scrunity and can open up excellent feasibility with various functionalities in opto-electronic devices. Here, we demonstrate that vertically stacked p-GaN/SiO/n-MoS/Graphene heterostructures enable to exhibit prominent dual opto-electronic characteristics, including efficient photo-detection and light emission, which represents the emergence of a new class of devices. The photoresponsivity was found to achieve as high as 10.4 AW and the detectivity and external quantum efficiency were estimated to be 1.1 × 10 Jones and ~30%, respectively. These values are superier than most reported hererojunction devices. In addition, this device exhibits as a self-powered photodetector, showing a high responsivity and fast response speed. Moreover, the device demonstrates the light emission with low turn-on voltage (1.0 V) which can be realized by electron injection from graphene electrode and holes from GaN film into monolayer MoS layer. These results indicate that with a suitable choice of band alignment, the vertical stacking of materials with different dimentionalities could be significant potential for integration of highly efficient heterostructures and open up feasible pathways towards integrated nanoscale multi-functional optoelectronic devices for a variety of applications.

摘要

将不同维度的材料集成在垂直堆叠的 p-n 异质结上引起了相当大的关注,并为光电设备中的各种功能开辟了极好的可行性。在这里,我们证明了垂直堆叠的 p-GaN/SiO/n-MoS2/Graphene 异质结构能够表现出突出的双光电特性,包括高效光电探测和发光,这代表了一类新设备的出现。发现光响应率高达10.4 AW,探测率和外量子效率估计分别为 1.1×10 琼斯和约 30%。这些值优于大多数报道的异质结设备。此外,该器件作为自供电光电探测器,表现出高响应率和快速响应速度。此外,该器件还表现出低开启电压(1.0 V)的发光,这可以通过从石墨烯电极注入电子和从 GaN 薄膜注入到单层 MoS 层的空穴来实现。这些结果表明,通过选择合适的能带排列,不同维度材料的垂直堆叠对于集成高效异质结构具有重要潜力,并为各种应用的集成纳米级多功能光电设备开辟了可行途径。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/951e/5577265/25317231f3c1/41598_2017_9998_Fig1_HTML.jpg

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