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相互作用的有机极化激元的高速流动。

High-speed flow of interacting organic polaritons.

作者信息

Lerario Giovanni, Ballarini Dario, Fieramosca Antonio, Cannavale Alessandro, Genco Armando, Mangione Federica, Gambino Salvatore, Dominici Lorenzo, De Giorgi Milena, Gigli Giuseppe, Sanvitto Daniele

机构信息

CNR NANOTEC -Istituto di Nanotecnologia, Via Monteroni, 73100 Lecce, Italy.

Dipartimento di matematica e fisica 'Ennio De Giorgi', Università del Salento, 73100 Lecce, Italy.

出版信息

Light Sci Appl. 2017 Feb 24;6(2):e16212. doi: 10.1038/lsa.2016.212. eCollection 2017 Feb.

Abstract

The strong coupling of an excitonic transition with an electromagnetic mode results in composite quasi-particles called exciton polaritons, which have been shown to combine the best properties of their individual components in semiconductor microcavities. However, the physics and applications of polariton flows in organic materials and at room temperature are still unexplored because of the poor photon confinement in such structures. Here, we demonstrate that polaritons formed by the hybridization of organic excitons with a Bloch surface wave are able to propagate for hundreds of microns showing remarkable third-order nonlinear interactions upon high injection density. These findings pave the way for the study of organic nonlinear light-matter fluxes and for a technologically promising route of the realization of dissipation-less on-chip polariton devices operating at room temperature.

摘要

激子跃迁与电磁模式的强耦合产生了称为激子极化激元的复合准粒子,在半导体微腔中,它们已被证明能兼具其各组成部分的最佳特性。然而,由于此类结构中光子限制较差,有机材料中以及室温下极化激元流的物理性质和应用仍未得到探索。在此,我们证明,由有机激子与布洛赫表面波杂化形成的极化激元能够传播数百微米,在高注入密度下表现出显著的三阶非线性相互作用。这些发现为有机非线性光与物质通量的研究以及实现室温下无耗散片上极化激元器件这一具有技术前景的途径铺平了道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/af27/6062184/1d188aa69d0d/lsa2016212f1.jpg

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