X射线原子对分布函数方法的兴起：一系列幸运事件。
The rise of the X-ray atomic pair distribution function method: a series of fortunate events.
作者信息
Billinge Simon J L
机构信息
1 Department of Applied Physics and Applied Mathematics , Columbia University , New York , NY 10027 , USA.
2 Condensed Matter Physics and Materials Science Department , Brookhaven National Laboratory , Upton , NY 11973 , USA.
出版信息
Philos Trans A Math Phys Eng Sci. 2019 Jun 17;377(2147):20180413. doi: 10.1098/rsta.2018.0413.
Abstract
The atomic pair distribution function (PDF) technique is a powerful approach to gain quantitative insight into the structure of materials where the structural coherence extends only over a few nanometres. In this paper, I focus on PDF from synchrotron X-rays and describe what is the PDF and where it came from, as well as key moments on the journey that have contributed to its enormous recent growth and expanding impact in materials science today. Synchrotron X-ray sources played a starring role in this story. This article is part of the theme issue 'Fifty years of synchrotron science: achievements and opportunities'.
摘要
原子对分布函数（PDF）技术是一种强大的方法，可用于深入定量了解结构相干性仅延伸至几纳米的材料结构。在本文中，我将重点介绍同步加速器X射线的PDF，并描述什么是PDF及其来源，以及在其近期取得巨大发展并在当今材料科学中产生日益扩大影响的历程中的关键节点。同步加速器X射线源在这个故事中扮演了主角。本文是主题为“同步加速器科学五十年：成就与机遇”的一部分。
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Nat Commun. 2018 Jun 18;9(1):2375. doi: 10.1038/s41467-018-04830-4.
2
Local Environment of Terbium(III) Ions in Layered Nanocrystalline Zirconium(IV) Phosphonate-Phosphate Ion Exchange Materials.层状纳米晶膦酸锆（IV）-磷酸离子交换材料中铽（III）离子的局部环境
Inorg Chem. 2017 Aug 7;56(15):8837-8846. doi: 10.1021/acs.inorgchem.7b00666. Epub 2017 Jul 13.
3
Towards atomistic understanding of polymorphism in the solvothermal synthesis of ZrO nanoparticles.迈向对ZrO纳米颗粒溶剂热合成中多晶型现象的原子层面理解。
Acta Crystallogr A Found Adv. 2016 Nov 1;72(Pt 6):645-650. doi: 10.1107/S2053273316012675. Epub 2016 Oct 3.
4
Atomic electron tomography: 3D structures without crystals.原子电子断层扫描技术：无需晶体的三维结构。
Science. 2016 Sep 23;353(6306). doi: 10.1126/science.aaf2157.
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Acta Crystallogr A Found Adv. 2015 Nov;71(Pt 6):562-8. doi: 10.1107/S2053273315014473. Epub 2015 Sep 22.
6
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